Cited by 469Electrocatalysts for Energy ConversionCO2 Reduction Techniques and CatalystsHydrogen Storage and Materials

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Heteroatom-Doped Transition Metal Electrocatalysts for Hydrogen Evolution Reaction

Jin, Huanyu, Liu, Xin, Chen, Shuangming, Vasileff, Anthony, Li, Laiquan, Jiao, Yan, Song, Li, Zheng, Yao, Qiao, Shi-Zhang·2019·ACS Energy Letters

DOI 10.1021/acsenergylett.9b00348

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Abstract

Developing efficient and low-cost electrocatalysts for the hydrogen evolution reaction (HER) is important for clean energy systems. Non-noble transition metals are the most promising candidates for replacement of conventional Pt group catalysts for the HER. However, most non-noble metals show poor HER activity due to their intrinsic electronic structures. Herein, we use a multifaceted heteroatom doping method (nitrogen, sulfur, and phosphorus) to directly and continuously fine-tune the electronic structure and HER activity of non-noble metals without changing their chemical composition. As a proof-of-concept, a nitrogen and phosphorus dual-doped Ni catalyst is explored by precisely manipulating doping modes, revealing the best HER performance among all doped Ni catalysts tested. The doping-induced charge redistribution in the Ni metal significantly influences its catalytic performance for the HER in alkaline media, which is confirmed by merging theoretical calculation with synchrotron-based spectroscopy. The principle that can bridge the doping modes and HER activity of the doped catalysts is built with a volcano relationship.

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Authors: Jin, H., Liu, X., Chen, S., Vasileff, A., Li, L., Jiao, Y., Song, L., Zheng, Y., & Qiao, S.-Z.
Affiliations: The University of Adelaide (AU)
University of Science and Technology of China (CN)
Corresponding author: Zheng, Yao
Qiao, Shi-Zhang
ORCID: Jin, Huanyu
Liu, Xin
Chen, Shuangming
Vasileff, Anthony
Li, Laiquan
Jiao, Yan
Song, Li
Zheng, Yao
Qiao, Shi-Zhang
Venue: ACS Energy Letters
Publisher: American Chemical Society (ACS)
Published: 2019-02-26
Volume: 4
Issue: 4
Pages: 805-810
ISSN: 2380-8195 (ISSN-L)
DOI: 10.1021/acsenergylett.9b00348
OpenAlex: W2916738214
Cited by: 469
References: 39
Citations by year: 2026: 39 · 2025: 57 · 2024: 70 · 2023: 76 · 2022: 65 · 2021: 64 · 2020: 67 · 2019: 31
FWCI: 12.07
Type: journal article
Language: en
Open access: closed
Licence: doi.org/10.15223/policy-029 (stm-asf)
doi.org/10.15223/policy-037 (stm-asf)
doi.org/10.15223/policy-045 (stm-asf)
Locations: ACS Energy Letters (publishedVersion)
Adelaide Research & Scholarship (AR&S) (University of Adelaide) (submittedVersion)
Funders: Australian Research Council (DP160104866, DE160101163, FL170100154)
Topics: Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › Electrocatalysts for Energy Conversion
Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › CO2 Reduction Techniques and Catalysts
Physical Sciences › Materials Science › Materials Chemistry › Hydrogen Storage and Materials
Keywords: hydrogen evolution reaction, heteroatom doping, non-noble metal electrocatalysts, nickel catalysts, electronic structure modulation, charge redistribution, alkaline water electrolysis, volcano relationship, low-cost hydrogen production

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Heteroatom-Doped Transition Metal Electrocatalysts for Hydrogen Evolution Reaction

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