The DOI matches its Crossref record; 15 of the 15 references it cites were found in a registry or an index.
Anion and Cation Modulation in Metal Compounds for Bifunctional Overall Water Splitting
Abstract
As substitutes for precious cathodic Pt/C and anodic IrO2 in electrolytic water splitting cells, a bifunctional catalyst electrode (Fe- and O-doped Co2P grown on nickel foam) has been fabricated by manipulating the cations and anions of metal compounds. The modified catalyst electrode exhibits both superior HER and OER performances with high activity, favorable kinetics, and outstanding durability. The overall ability toward water splitting is especially extraordinary, requiring a small overpotential of 333.5 mV to gain a 10 mA cm(-2) current density. A study on the electrocatalytic mechanism reveals that the atomic modulation between cation and anion plays an important role in optimizing the electrocatalytic activity, which greatly expands the active sites in the electrocatalyst. Further, the three-dimensional conductive porous network is highly advantageous for the exposure of active species, the transport of bubble products, and the transfer of electrons and charges, which substantially boosts reaction kinetics and structure stability.
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Cites
Benchmarking Heterogeneous Electrocatalysts for the Oxygen Evolution Reaction
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Nanostructured Nickel Phosphide as an Electrocatalyst for the Hydrogen Evolution Reaction
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Cited by
Electrocatalysis for the oxygen evolution reaction: recent development and future perspectives
Suen, N.-T., Hung, S.-F., Quan, Q., Zhang, N., Xu, Y.-J., & Chen, H. M. (2017) · Chemical Society Reviews · doi:10.1039/c6cs00328a · Cited by 6,307
Non‐Noble Metal‐based Carbon Composites in Hydrogen Evolution Reaction: Fundamentals to Applications
Wang, J., Xu, F., Jin, H., Chen, Y., & Wang, Y. (2017) · Advanced Materials · doi:10.1002/adma.201605838 · Cited by 1,769
Wang, X., Liu, J., Liu, Z., Wang, W., Luo, J., Han, X., Du, X., Qiao, S., & Yang, J. (2018) · Advanced Materials · doi:10.1002/adma.201800005 · Cited by 640
Self-citationMultifunctional Transition Metal‐Based Phosphides in Energy‐Related Electrocatalysis
Li, Y., Dong, Z., & Jiao, L. (2020) · Advanced Energy Materials · doi:10.1002/aenm.201902104 · Cited by 603
Liang, H., Gandi, A. N., Xia, C., Hedhili, M. N., Anjum, D. H., Schwingenschlögl, U., & Alshareef, H. N. (2017) · ACS Energy Letters · doi:10.1021/acsenergylett.7b00206 · Cited by 588
Metadata
- Authors
- Duan, J., Chen, S., Vasileff, A., & Qiao, S. Z.
- Venue
- ACS Nano
- Publisher
- American Chemical Society (ACS)
- Published
- 2016-09-15
- Volume
- 10
- Issue
- 9
- Pages
- 8738-8745
- ISSN
- 1936-0851 (ISSN-L)
- 1936-086X
- OpenAlex
- W2519334698
- Cited by
- 409
- References
- 15
- FWCI
- 17.34
- Type
- journal article
- Language
- en
- Open access
- closed
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