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Atomic H-Induced Mo2C Hybrid as an Active and Stable Bifunctional Electrocatalyst
Open accessAbstract
Mo 2 C nanocrystals (NCs) anchored on vertically aligned graphene nanoribbons (VA-GNR) as hybrid nanoelectrocatalysts (Mo 2 C–GNR) are synthesized through the direct carbonization of metallic Mo with atomic H treatment. The growth mechanism of Mo 2 C NCs with atomic H treatment is discussed. The Mo 2 C–GNR hybrid exhibits highly active and durable electrocatalytic performance for the hydrogen-evolution reaction (HER) and oxygen-reduction reaction (ORR). For HER, in an acidic solution the Mo 2 C–GNR has an onset potential of 39 mV and a Tafel slope of 65 mV dec –1, and in a basic solution Mo 2 C–GNR has an onset potential of 53 mV, and Tafel slope of 54 mV dec –1 . It is stable in both acidic and basic media. Mo 2 C–GNR is a high-activity ORR catalyst with a high peak current density of 2.01 mA cm –2, an onset potential of 0.93 V that is more positive vs reversible hydrogen electrode (RHE), a high electron transfer number n (∼3.90), and long-term stability.
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Cites
Benchmarking Heterogeneous Electrocatalysts for the Oxygen Evolution Reaction
McCrory, C. C. L., Jung, S., Peters, J. C., & Jaramillo, T. F. (2013) · Journal of the American Chemical Society · doi:10.1021/ja407115p · Cited by 7,026
MoS 2 Nanoparticles Grown on Graphene: An Advanced Catalyst for the Hydrogen Evolution Reaction
Li, Y., Wang, H., Xie, L., Liang, Y., Hong, G., & Dai, H. (2011) · Journal of the American Chemical Society · doi:10.1021/ja201269b · Cited by 5,001
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Cited by
Gao, Q., Zhang, W., Shi, Z., Yang, L., & Tang, Y. (2019) · Advanced Materials · doi:10.1002/adma.201802880 · Cited by 734
Luo, Y., Tang, L., Khan, U., Yu, Q., Cheng, H.-M., Zou, X., & Liu, B. (2019) · Nature Communications · doi:10.1038/s41467-018-07792-9 · Cited by 713
Wang, R., Dong, X., Du, J., Zhao, J., & Zang, S. (2018) · Advanced Materials · doi:10.1002/adma.201703711 · Cited by 580
Jia, J., Xiong, T., Zhao, L., Wang, F., Liu, H., Hu, R., Zhou, J., Zhou, W., & Chen, S. (2017) · ACS Nano · doi:10.1021/acsnano.7b06607 · Cited by 470
Heterostructures of MXenes and N-doped graphene as highly active bifunctional electrocatalysts
Zhou, S., Yang, X., Pei, W., Liu, N., & Zhao, J. (2018) · Nanoscale · doi:10.1039/c8nr01090k · Cited by 282
Metadata
- Authors
- Fan, X., Liu, Y., Peng, Z., Zhang, Z., Zhou, H., Zhang, X., Yakobson, B. I., Goddard, W. A., Guo, X., Hauge, R. H., & Tour, J. M.
- Venue
- ACS Nano
- Publisher
- American Chemical Society (ACS)
- Published
- 2017-01-03
- Volume
- 11
- Issue
- 1
- Pages
- 384-394
- ISSN
- 1936-0851 (ISSN-L)
- 1936-086X
- OpenAlex
- W2564996136
- Cited by
- 158
- References
- 4
- FWCI
- 6.08
- Type
- journal article
- Language
- en
- Open access
- green
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- Fan, X., Liu, Y., Peng, Z., Zhang, Z., Zhou, H., Zhang, X., Yakobson, B. I., Goddard, W. A., Guo, X., Hauge, R. H., & Tour, J. M. (2017). Atomic H-Induced Mo2C Hybrid as an Active and Stable Bifunctional Electrocatalyst. ACS Nano. https://doi.org/10.1021/acsnano.6b06089
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