The DOI matches its Crossref record; 104 of the 104 references it cites were found in a registry or an index.
MOF‐Derived Bifunctional Cu3P Nanoparticles Coated by a N,P‐Codoped Carbon Shell for Hydrogen Evolution and Oxygen Reduction
Abstract
Metal–organic frameworks (MOFs) have recently emerged as a type of uniformly and periodically atom‐distributed precursor and efficient self‐sacrificial template to fabricate hierarchical porous‐carbon‐related nanostructured functional materials. For the first time, a Cu‐based MOF, i.e., Cu‐NPMOF is used, whose linkers contain nitrogen and phosphorus heteroatoms, as a single precursor and template to prepare novel Cu 3 P nanoparticles (NPs) coated by a N,P‐codoped carbon shell that is extended to a hierarchical porous carbon matrix with identical uniform N and P doping (termed Cu 3 P@NPPC) as an electrocatalyst. Cu 3 P@NPPC demonstrates outstanding activity for both the hydrogen evolution and oxygen reduction reaction, representing the first example of a Cu 3 P‐based bifunctional catalyst for energy‐conversion reactions. The high performances are ascribed to the high specific surface area, the synergistic effects of the Cu 3 P NPs with intrinsic activity, the protection of the carbon shell, and the hierarchical porous carbon matrix doped by multiheteroatoms. This strategy of using a diverse MOF as a structural and compositional material to create a new multifunctional composite/hybrid may expand the opportunities to explore highly efficient and robust non‐noble‐metal catalysts for energy‐conversion reactions.
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Cited by
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Metadata
- Authors
- Wang, R., Dong, X., Du, J., Zhao, J., & Zang, S.
- Venue
- Advanced Materials
- Publisher
- Wiley
- Published
- 2017-12-21
- Volume
- 30
- Issue
- 6
- ISSN
- 0935-9648 (ISSN-L)
- 1521-4095
- OpenAlex
- W2776776548
- Cited by
- 580
- References
- 104
- FWCI
- 20.78
- Type
- journal article
- Language
- en
- Open access
- closed
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