The DOI matches its Crossref record; 9 of the 9 references it cites were found in a registry or an index.
Fluorine Doped Cagelike Carbon Electrocatalyst: An Insight into the Structure-Enhanced CO Selectivity for CO2 Reduction at High Overpotential
Abstract
The critical bottleneck of electrocatalytic CO 2 reduction reaction (CO 2 RR) lies in its low efficiency at high overpotential caused by competitive hydrogen evolution. It is challenging to develop an efficient catalyst achieving both high current density and high Faradaic efficiency (FE) for CO 2 RR. Herein, we synthesized fluorine-doped cagelike porous carbon (F-CPC) by purposely tailoring its structural properties. The optimized F-CPC possesses large surface area with moderate mesopore and abundant micropores as well as high electrical conductivity. When used as catalyst for CO 2 RR, F-CPC exhibits FE of 88.3% for CO at −1.0 V vs RHE with a current density of 37.5 mA·cm –2 . Experimental results and finite element simulations demonstrate that the excellent CO 2 RR performance of F-CPC at high overpotential should be attributed to its structure-enhanced electrocatalytic process stemming from its cagelike morphology.
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Cites
Enhanced electrocatalytic CO2 reduction via field-induced reagent concentration
Liu, M., Pang, Y., Zhang, B., De Luna, P., Voznyy, O., Xu, J., Zheng, X., Dinh, C. T., Fan, F., Cao, C., et al. (2016) · Nature · doi:10.1038/nature19060 · Cited by 2,000
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Partially oxidized atomic cobalt layers for carbon dioxide electroreduction to liquid fuel
Gao, S., Lin, Y., Jiao, X., Sun, Y., Luo, Q., Zhang, W., Li, D., Yang, J., & Xie, Y. (2016) · Nature · doi:10.1038/nature16455 · Cited by 1,865
Recent Advances in Inorganic Heterogeneous Electrocatalysts for Reduction of Carbon Dioxide
Zhu, D. D., Liu, J. L., & Qiao, S. Z. (2016) · Advanced Materials · doi:10.1002/adma.201504766 · Cited by 1,594
Liu, D., Li, X., Chen, S., Yan, H., Wang, C., Wu, C., Haleem, Y. A., Duan, S., Lu, J., Ge, B., et al. (2019) · Nature Energy · doi:10.1038/s41560-019-0402-6 · Cited by 1,166
Hoang, T. T. H., Verma, S., Ma, S., Fister, T. T., Timoshenko, J., Frenkel, A. I., Kenis, P. J. A., & Gewirth, A. A. (2018) · Journal of the American Chemical Society · doi:10.1021/jacs.8b01868 · Cited by 852
Jiang, B., Zhang, X.-G., Jiang, K., Wu, D.-Y., & Cai, W.-B. (2018) · Journal of the American Chemical Society · doi:10.1021/jacs.7b12506 · Cited by 402
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Cited by
Electrocatalysis for CO 2 conversion: from fundamentals to value-added products
Wang, G., Chen, J., Ding, Y., Cai, P., Yi, L., Li, Y., Tu, C., Hou, Y., Wen, Z., & Dai, L. (2021) · Chemical Society Reviews · doi:10.1039/d0cs00071j · Cited by 1,295
Li, Y., Li, B., Zhang, D., Cheng, L., & Xiang, Q. (2020) · ACS Nano · doi:10.1021/acsnano.0c04544 · Cited by 666
Gong, S., Xiao, X., Wang, W., Sam, D. K., Lu, R., Xu, Y., Liu, J., Wu, C., & Lv, X. (2021) · Journal of Colloid and Interface Science · doi:10.1016/j.jcis.2021.05.054 · Cited by 42
Metadata
- Authors
- Ni, W., Xue, Y., Zang, X., Li, C., Wang, H., Yang, Z., & Yan, Y.-M.
- Venue
- ACS Nano
- Publisher
- American Chemical Society (ACS)
- Published
- 2020-02-12
- Volume
- 14
- Issue
- 2
- Pages
- 2014-2023
- ISSN
- 1936-0851 (ISSN-L)
- 1936-086X
- OpenAlex
- W3006017306
- Cited by
- 183
- References
- 9
- FWCI
- 5.11
- Type
- journal article
- Language
- en
- Open access
- closed
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