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Highly Adhesive Li-BN Nanosheet Composite Anode with Excellent Interfacial Compatibility for Solid-State Li Metal Batteries
Abstract
Abstract Solid-state lithium metal batteries (SSLMBs) are promising energy storage devices by employing lithium metal anodes and solid-state electrolytes (SSEs) to offer high energy density and high safety. However, their efficiency is limited by Li metal/SSE interface barriers, including insufficient contact area and chemical/electrochemical incompatibility. Herein, a strategy to effectively improve the adhesiveness of Li metal to garnet-type SSE is proposed by adding only a few two-dimensional boron nitride nanosheets (BNNS) (5 wt %) into Li metal by triggering the transition from point contact to complete adhesion between Li metal and ceramic SSE. The interface between the Li-BNNS composite anode and the garnet exhibits a low interfacial resistance of 9 Ω cm2, which is significantly lower than that of bare Li/garnet interface (560 Ω cm2). Furthermore, the enhanced contact and the additional BNNS in the interface act synergistically to offer a high critical current density of 1.5 mA/cm2 and a stable electrochemical plating/striping over 380 h. Moreover, the full cell paired with the Li-BNNS composite anode and the LiFePO4 cathode shows stable cycling performance at room temperature. Our results introduce an appealing composite strategy with two-dimensional materials to overcome the interface challenges, which provide more opportunities for the development of SSLMBs.
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Citations
Cites
Reviving the lithium metal anode for high-energy batteries
Lin, D., Liu, Y., & Cui, Y. (2017) · Nature Nanotechnology · doi:10.1038/nnano.2017.16 · Cited by 6,763
Cited by
Confronting the Challenges in Lithium Anodes for Lithium Metal Batteries
Wang, Q., Liu, B., Shen, Y., Wu, J., Zhao, Z., Zhong, C., & Hu, W. (2021) · Advanced Science · doi:10.1002/advs.202101111 · Cited by 531
Reducing the thickness of solid-state electrolyte membranes for high-energy lithium batteries
Wu, J., Yuan, L., Zhang, W., Li, Z., Xie, X., & Huang, Y. (2021) · Energy & Environmental Science · doi:10.1039/d0ee02241a · Cited by 425
Self-citationZhao, F., Sun, Q., Yu, C., Zhang, S., Adair, K., Wang, S., Liu, Y., Zhao, Y., Liang, J., Wang, C., et al. (2020) · ACS Energy Letters · doi:10.1021/acsenergylett.0c00207 · Cited by 294
Strategies to anode protection in lithium metal battery: A review
Li, J., Kong, Z., Liu, X., Zheng, B., Fan, Q. H., Garratt, E., Schuelke, T., Wang, K., Xu, H., & Jin, H. (2021) · InfoMat · doi:10.1002/inf2.12189 · Cited by 267
Metadata
- Authors
- Wen, J., Huang, Y., Duan, J., Wu, Y., Luo, W., Zhou, L., Hu, C., Huang, L., Zheng, X., Yang, W., Wen, Z., & Huang, Y.
- Venue
- ACS Nano
- Publisher
- American Chemical Society (ACS)
- Published
- 2019-12-02
- Volume
- 13
- Issue
- 12
- Pages
- 14549-14556
- ISSN
- 1936-0851 (ISSN-L)
- 1936-086X
- OpenAlex
- W2990482559
- Cited by
- 160
- References
- 1
- FWCI
- 7.49
- Type
- journal article
- Language
- en
- Open access
- closed
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- Wen, J., Huang, Y., Duan, J., Wu, Y., Luo, W., Zhou, L., Hu, C., Huang, L., Zheng, X., Yang, W., Wen, Z., & Huang, Y. (2019). Highly Adhesive Li-BN Nanosheet Composite Anode with Excellent Interfacial Compatibility for Solid-State Li Metal Batteries. ACS Nano. https://doi.org/10.1021/acsnano.9b08803
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