The DOI matches its Crossref record; 46 of the 46 references it cites were found in a registry or an index.
Ti3C2Tx MXene-Reduced Graphene Oxide Composite Electrodes for Stretchable Supercapacitors
Abstract
The development of stretchable electronics requires the invention of compatible high-performance power sources, such as stretchable supercapacitors and batteries. In this work, two-dimensional (2D) titanium carbide (Ti 3 C 2 T x ) MXene is being explored for flexible and printed energy storage devices by fabrication of a robust, stretchable high-performance supercapacitor with reduced graphene oxide (RGO) to create a composite electrode. The Ti 3 C 2 T x /RGO composite electrode combines the superior electrochemical and mechanical properties of Ti 3 C 2 T x and the mechanical robustness of RGO resulting from strong nanosheet interactions, larger nanoflake size, and mechanical flexibility. It is found that the Ti 3 C 2 T x /RGO composite electrodes with 50 wt % RGO incorporated prove to mitigate cracks generated under large strains. The composite electrodes exhibit a large capacitance of 49 mF/cm 2 (∼490 F/cm 3 and ∼140 F/g) and good electrochemical and mechanical stability when subjected to cyclic uniaxial (300%) or biaxial (200% × 200%) strains. The as-assembled symmetric supercapacitor demonstrates a specific capacitance of 18.6 mF/cm 2 (∼90 F/cm 3 and ∼29 F/g) and a stretchability of up to 300%. The developed approach offers an alternative strategy to fabricate stretchable MXene-based energy storage devices and can be extended to other members of the large MXene family.
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Citations
Cites
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2D metal carbides and nitrides (MXenes) for energy storage
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Self-citationElectromagnetic interference shielding with 2D transition metal carbides (MXenes)
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Self-citationFully integrated wearable sensor arrays for multiplexed in situ perspiration analysis
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Two-Dimensional Transition Metal Carbides
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Self-citationSkin-like pressure and strain sensors based on transparent elastic films of carbon nanotubes
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Ultra-high-rate pseudocapacitive energy storage in two-dimensional transition metal carbides
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Self-citationFlexible and conductive MXene films and nanocomposites with high capacitance
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Two-Dimensional, Ordered, Double Transition Metals Carbides (MXenes)
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Cited by
Lu, Y., Fan, D., Wang, Y., Xu, H., Lu, C., & Yang, X. (2021) · ACS Nano · doi:10.1021/acsnano.1c02578 · Cited by 426
Metadata
- Authors
- Zhou, Y., Maleski, K., Anasori, B., Thostenson, J. O., Pang, Y., Feng, Y., Zeng, K., Parker, C. B., Zauscher, S., Gogotsi, Y., Glass, J. T., & Cao, C.
- Venue
- ACS Nano
- Publisher
- American Chemical Society (ACS)
- Published
- 2020-02-12
- Volume
- 14
- Issue
- 3
- Pages
- 3576-3586
- ISSN
- 1936-0851 (ISSN-L)
- 1936-086X
- OpenAlex
- W3006668308
- Cited by
- 459
- References
- 46
- FWCI
- 24.80
- Type
- journal article
- Language
- en
- Open access
- closed
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- Zhou, Y., Maleski, K., Anasori, B., Thostenson, J. O., Pang, Y., Feng, Y., Zeng, K., Parker, C. B., Zauscher, S., Gogotsi, Y., Glass, J. T., & Cao, C. (2020). Ti3C2Tx MXene-Reduced Graphene Oxide Composite Electrodes for Stretchable Supercapacitors. ACS Nano. https://doi.org/10.1021/acsnano.9b10066
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