The DOI matches its Crossref record; 3 of the 3 references it cites were found in a registry or an index.
Two-Dimensional Transition Metal Carbides
Abstract
Herein we report on the synthesis of two-dimensional transition metal carbides and carbonitrides by immersing select MAX phase powders in hydrofluoric acid, HF. The MAX phases represent a large (>60 members) family of ternary, layered, machinable transition metal carbides, nitrides, and carbonitrides. Herein we present evidence for the exfoliation of the following MAX phases: Ti(2)AlC, Ta(4)AlC(3), (Ti(0.5),Nb(0.5))(2)AlC, (V(0.5),Cr(0.5))(3)AlC(2), and Ti(3)AlCN by the simple immersion of their powders, at room temperature, in HF of varying concentrations for times varying between 10 and 72 h followed by sonication. The removal of the "A" group layer from the MAX phases results in 2-D layers that we are labeling MXenes to denote the loss of the A element and emphasize their structural similarities with graphene. The sheet resistances of the MXenes were found to be comparable to multilayer graphene. Contact angle measurements with water on pressed MXene surfaces showed hydrophilic behavior.
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Citations
Cites
Electric Field Effect in Atomically Thin Carbon Films
Novoselov, K. S., Geim, A. K., Morozov, S. V., Jiang, D., Zhang, Y., Dubonos, S. V., Grigorieva, I. V., & Firsov, A. A. (2004) · Science · doi:10.1126/science.1102896 · Cited by 66,834
Graphene-based composite materials
Stankovich, S., Dikin, D. A., Dommett, G. H. B., Kohlhaas, K. M., Zimney, E. J., Stach, E. A., Piner, R. D., Nguyen, S. T., & Ruoff, R. S. (2006) · Nature · doi:10.1038/nature04969 · Cited by 12,922
Two-dimensional atomic crystals
Novoselov, K. S., Jiang, D., Schedin, F., Booth, T. J., Khotkevich, V. V., Morozov, S. V., & Geim, A. K. (2005) · Proceedings of the National Academy of Sciences · doi:10.1073/pnas.0502848102 · Cited by 11,788
Cited by
Xie, Y., Naguib, M., Mochalin, V. N., Barsoum, M. W., Gogotsi, Y., Yu, X., Nam, K.-W., Yang, X.-Q., Kolesnikov, A. I., & Kent, P. R. C. (2014) · Journal of the American Chemical Society · doi:10.1021/ja501520b · Cited by 1,537
Self-citationTwo-Dimensional Molybdenum Carbide (MXene) as an Efficient Electrocatalyst for Hydrogen Evolution
Seh, Z. W., Fredrickson, K. D., Anasori, B., Kibsgaard, J., Strickler, A. L., Lukatskaya, M. R., Gogotsi, Y., Jaramillo, T. F., & Vojvodic, A. (2016) · ACS Energy Letters · doi:10.1021/acsenergylett.6b00247 · Cited by 1,482
Self-citationTwo-Dimensional Ultrathin MXene Ceramic Nanosheets for Photothermal Conversion
Lin, H., Wang, X., Yu, L., Chen, Y., & Shi, J. (2017) · Nano Letters · doi:10.1021/acs.nanolett.6b04339 · Cited by 1,314
Ten Years of Progress in the Synthesis and Development of MXenes
Naguib, M., Barsoum, M. W., & Gogotsi, Y. (2021) · Advanced Materials · doi:10.1002/adma.202103393 · Cited by 1,257
Self-citation2D MXenes: A New Family of Promising Catalysts for the Hydrogen Evolution Reaction
Gao, G., O’Mullane, A. P., & Du, A. (2017) · ACS Catalysis · doi:10.1021/acscatal.6b02754 · Cited by 1,153
Metadata
- Authors
- Naguib, M., Mashtalir, O., Carle, J., Presser, V., Lu, J., Hultman, L., Gogotsi, Y., & Barsoum, M. W.
- Venue
- ACS Nano
- Publisher
- American Chemical Society (ACS)
- Published
- 2012-02-13
- Volume
- 6
- Issue
- 2
- Pages
- 1322-1331
- ISSN
- 1936-0851 (ISSN-L)
- 1936-086X
- OpenAlex
- W1981729886
- Cited by
- 4,769
- References
- 3
- FWCI
- 26.06
- Type
- journal article
- Language
- en
- Open access
- closed
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- Naguib, M., Mashtalir, O., Carle, J., Presser, V., Lu, J., Hultman, L., Gogotsi, Y., & Barsoum, M. W. (2012). Two-Dimensional Transition Metal Carbides. ACS Nano. https://doi.org/10.1021/nn204153h
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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