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Performance Comparison of Proton Exchange Membrane Fuel Cells with Nafion and Aquivion Perfluorosulfonic Acids with Different Equivalent Weights as the Electrode Binders
Open accessAbstract
A perfluorosulfonic acid (PFSA) ionomer, used as the proton conductor in the catalyst layer, influences significantly the performance of proton exchange membrane fuel cell catalyst-coated membrane (CCM). In this paper, SSC-CCM is prepared by the SSC-PFSA (Aquivion, EW 720) ionomer, and the comparative sample (LSC-CCM) is based on the LSC-PFSA ionomer (Nafion, EW 1100). Compared with LSC-CCM, SSC-CCM shows higher porosity, larger electrochemical surface area (ECSA), and smaller high-frequency resistance. Polarization curves of SSC-CCM tested by the short stack show better performance than those of LSC-CCM, especially under the lower relative humidity operations. Moreover, the SSC-CCM outputs higher voltage and is more stable in the dynamic process with temperature continuously increasing under lower relative humidity operation. Such excellent performance of SSC-CCM is confirmed from the higher proton conductivity of SSC-PFSA under low relative humidity. These results indicate that the SSC-PFSA ionomer could be employed for the CCM catalyst layer under the operation conditions of low relative humidity and dynamic running for automotive applications.
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Aquivion SSC membranes show higher ionic conductivity, higher water absorption, similar mechanical properties, and higher glass transition than Nafion LSC membranes.
“Compared with the Nafion LSC membrane, Aquivion SSC membranes show higher ionic conductivity, higher water absorption, similar mechanical properties, and higher glass transition [78]”
From Recent Advances on PEM Fuel Cells: From Key Materials to Membrane Electrode Assembly (2023) · cites this paper as [78]
The Results and Discussion section (“Water Uptake and Proton Conductivity”; page unavailable) reports higher water uptake and proton conductivity for Aquivion SSC-720 than for Nafion LSC-1100 under the tested conditions, although their conductivities were similar at 20% relative humidity. The Introduction (page unavailable) reports a higher glass-transition temperature for Aquivion at a given equivalent weight. The paper does not report that the membranes have similar mechanical properties. (LLM, conf=0.88)
Experimental — accuracy not yet measuredAquivion SSC membranes present better performance in MEA, particularly at low humidity, compared with Nafion LSC membranes.
“to therefore present better performance in MEA, particularly at low humidity (Fig. 5c).”
From Recent Advances on PEM Fuel Cells: From Key Materials to Membrane Electrode Assembly (2023) · cites this paper as [78]
The Results and Discussion section (Static Performance Response to Operation Conditions; page not provided) reports better performance for Aquivion-based SSC-CCMs than Nafion-based LSC-CCMs, with the difference greatest at low humidity. But the Experimental Section (Preparation of CCM; page not provided) says both were made by spraying different electrode-binder ionomers onto the same Gore membrane. The study therefore does not establish that an Aquivion membrane outperforms a Nafion membrane in an MEA. (LLM, conf=0.90)
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Metadata
- Authors
- Li, T., Shen, J., Chen, G., Guo, S., & Xie, G.
- Affiliations
- Sichuan University (CN)
- Dongfang Electric Corporation (China) (CN)
- Corresponding author
- Guo, Shaoyun
- Xie, Guangyou
- Venue
- ACS Omega
- Publisher
- American Chemical Society (ACS)
- Published
- 2020-07-07
- Volume
- 5
- Issue
- 28
- Pages
- 17628-17636
- ISSN
- 2470-1343 (ISSN-L)
- PMC
- PMC7377320
- OpenAlex
- W3040968267
- Cited by
- 81
- References
- 33
- Citations by year
- 2026: 23 · 2025: 12 · 2024: 14 · 2023: 10 · 2022: 11 · 2021: 11
- FWCI
- 2.75
- Type
- journal article
- Language
- en
- Open access
- gold
- doi.org
- Licence
- Locations
- ACS Omega (publishedVersion, other-oa)
- PubMed Central (publishedVersion)
- PubMed (publishedVersion)
- DOAJ (DOAJ: Directory of Open Access Journals) (submittedVersion, cc-by-sa)
- Funders
- Ministry of Science and Technology of the People's Republic of China (2018YFB1502505)
- Sichuan Province (2016GZ0027, 2017CC0017)
- Topics
- Physical Sciences › Engineering › Electrical and Electronic Engineering › Fuel Cells and Related Materials
- Physical Sciences › Materials Science › Materials Chemistry › Advancements in Solid Oxide Fuel Cells
- Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › Electrocatalysts for Energy Conversion
- Keywords
- proton exchange membrane fuel cells, perfluorosulfonic acid ionomer, Aquivion, Nafion, equivalent weight, catalyst coated membranes, electrode binder, low relative humidity operation, proton conductivity, electrochemically active surface area, membrane porosity, automotive fuel cells
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