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Magnetic Alignment of Hexagonal Boron Nitride Platelets in Polymer Matrix: Toward High Performance Anisotropic Polymer Composites for Electronic Encapsulation
Abstract
We report magnetic alignment of hexagonal boron nitride (hBN) platelets and the outstanding material properties of its polymer composite. The magnetically responsive hBN is produced by surface modification of iron oxide, and their orientations can be controlled by applying an external magnetic field during polymer curing. Owing to the anisotropic properties of hBN, the epoxy composite with aligned hBN platelets shows interesting properties along the alignment direction, including significantly reduced coefficient of thermal expansion, reaching ∼28.7 ppm/°C, and enhanced thermal conductivity, 104% higher than that of unaligned counterpart, both of which are observed at a low filler loading of 20 wt %. Our modeling suggests the filler alignment is the major reason for these intriguing material properties. Finite element analysis reveals promising applications for the magnetically aligned hBN-based composites in modern microelectronic packaging.
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Cites
Graphene–Multilayer Graphene Nanocomposites as Highly Efficient Thermal Interface Materials
Shahil, K. M. F., & Balandin, A. A. (2012) · Nano Letters · doi:10.1021/nl203906r · Cited by 1,467
Thermal Interface Materials: Historical Perspective, Status, and Future Directions
Prasher, R. (2006) · Proceedings of the IEEE · doi:10.1109/jproc.2006.879796 · Cited by 927
Cited by
Hu, J., Huang, Y., Yao, Y., Pan, G., Sun, J., Zeng, X., Sun, R., Xu, J.-B., Song, B., & Wong, C.-P. (2017) · ACS Applied Materials & Interfaces · doi:10.1021/acsami.7b02410 · Cited by 499
Self-citationConstruction of 3D Skeleton for Polymer Composites Achieving a High Thermal Conductivity
Yao, Y., Sun, J., Zeng, X., Sun, R., Xu, J., & Wong, C. (2018) · Small · doi:10.1002/smll.201704044 · Cited by 389
Self-citationLian, G., Tuan, C.-C., Li, L., Jiao, S., Wang, Q., Moon, K.-S., Cui, D., & Wong, C.-P. (2016) · Chemistry of Materials · doi:10.1021/acs.chemmater.6b01595 · Cited by 382
Self-citationYang, J., Tang, L.-S., Bai, L., Bao, R.-Y., Liu, Z.-Y., Xie, B.-H., Yang, M.-B., & Yang, W. (2019) · Materials Horizons · doi:10.1039/c8mh01219a · Cited by 269
Yang, J., Tang, L.-S., Bai, L., Bao, R.-Y., Liu, Z., Xie, B.-H., Yang, M.-B., & Yang, W. (2018) · ACS Sustainable Chemistry & Engineering · doi:10.1021/acssuschemeng.8b00565 · Cited by 105
Metadata
- Authors
- Lin, Z., Liu, Y., Raghavan, S., Moon, K.-S., Sitaraman, S. K., & Wong, C.-P.
- Venue
- ACS Applied Materials & Interfaces
- Publisher
- American Chemical Society (ACS)
- Published
- 2013-07-15
- Volume
- 5
- Issue
- 15
- Pages
- 7633-7640
- ISSN
- 1944-8244 (ISSN-L)
- 1944-8252
- OpenAlex
- W2319155157
- Cited by
- 469
- References
- 2
- FWCI
- 7.10
- Type
- journal article
- Language
- en
- Open access
- closed
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- Lin, Z., Liu, Y., Raghavan, S., Moon, K.-S., Sitaraman, S. K., & Wong, C.-P. (2013). Magnetic Alignment of Hexagonal Boron Nitride Platelets in Polymer Matrix: Toward High Performance Anisotropic Polymer Composites for Electronic Encapsulation. ACS Applied Materials & Interfaces. https://doi.org/10.1021/am401939z
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