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Facile Fabrication of Highly Efficient g-C3N4/Ag2O Heterostructured Photocatalysts with Enhanced Visible-Light Photocatalytic Activity
Abstract
Highly efficient visible-light-driven g-C3N4/Ag2O heterostructured photocatalysts were prepared by a simple liquid phase synthesis method at room temperature. The composition, structure, morphology, and optical absorption properties of the as-prepared g-C3N4/Ag2O composites were characterized by XRD, FTIR, XPS, TEM, and UV-vis DRS, respectively. We found interestingly that the photogenerated charge carriers separations of the as-prepared g-C3N4/Ag2O composites were closely related to the mass ratio of g-C3N4 and Ag2O. When the mass ratio of g-C3N4 and Ag2O reached 1:4, the as-prepared composite exhibited the highest photocatalytic activity, which was almost 11 and 1.2 times as high as that of individual g-C3N4 and Ag2O, respectively. The enhancement of photocatalytic activity could be attributed to the synergetic effects between g-C3N4 and Ag2O as well as the improved dispersibility and the decreased particle size of Ag2O. Moreover, the as-prepared composites showed excellent stability toward the photodegradation of methyl orange (MO). Finally, a possible photocatalytic and charge separation mechanism was proposed.
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Metadata
- Authors
- Xu, M., Han, L., & Dong, S.
- Venue
- ACS Applied Materials & Interfaces
- Publisher
- American Chemical Society (ACS)
- Published
- 2013-11-19
- Volume
- 5
- Issue
- 23
- Pages
- 12533-12540
- ISSN
- 1944-8244 (ISSN-L)
- 1944-8252
- OpenAlex
- W2313200550
- Cited by
- 594
- References
- 40
- FWCI
- 17.55
- Type
- journal article
- Language
- en
- Open access
- closed
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