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In Situ Ion Exchange Synthesis of Strongly Coupled Ag@AgCl/g-C3N4 Porous Nanosheets as Plasmonic Photocatalyst for Highly Efficient Visible-Light Photocatalysis
Abstract
A novel efficient Ag@AgCl/g-C3N4 plasmonic photocatalyst was synthesized by a rational in situ ion exchange approach between exfoliated g-C3N4 nanosheets with porous 2D morphology and AgNO3. The as-prepared Ag@AgCl-9/g-C3N4 plasmonic photocatalyst exhibited excellent photocatalytic performance under visible light irradiation for rhodamine B degradation with a rate constant of 0.1954 min(-1), which is ∼41.6 and ∼16.8 times higher than those of the g-C3N4 (∼0.0047 min(-1)) and Ag/AgCl (∼0.0116 min(-1)), respectively. The degradation of methylene blue, methyl orange, and colorless phenol further confirmed the broad spectrum photocatalytic degradation abilities of Ag@AgCl-9/g-C3N4. These results suggested that an integration of the synergetic effect of suitable size plasmonic Ag@AgCl and strong coupling effect between the Ag@AgCl nanoparticles and the exfoliated porous g-C3N4 nanosheets was superior for visible-light-responsive and fast separation of photogenerated electron-hole pairs, thus significantly improving the photocatalytic efficiency. This work may provide a novel concept for the rational design of stable and high performance g-C3N4-based plasmonic photocatalysts for unique photochemical reaction.
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Metadata
- Authors
- Zhang, S., Li, J., Wang, X., Huang, Y., Zeng, M., & Xu, J.
- Venue
- ACS Applied Materials & Interfaces
- Publisher
- American Chemical Society (ACS)
- Published
- 2014-12-04
- Volume
- 6
- Issue
- 24
- Pages
- 22116-22125
- ISSN
- 1944-8244 (ISSN-L)
- 1944-8252
- OpenAlex
- W2325112411
- Cited by
- 432
- References
- 38
- FWCI
- 15.61
- Type
- journal article
- Language
- en
- Open access
- closed
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