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Production of Bioactive Cellulose Films Reconstituted from Ionic Liquids
Abstract
A new method for introducing enzymes into cellulosic matrixes which can be formed into membranes, films, or beads has been developed using a cellulose-in-ionic-liquid dissolution and regeneration process. Initial results on the formation of thin cellulose films incorporating dispersed laccase indicate that active enzyme-encapsulated films can be prepared using this methodology and that precoating the enzyme with a second, hydrophobic ionic liquid prior to dispersion in the cellulose/ionic liquid solution can provide an increase in enzyme activity relative to that of untreated films, presumably by providing a stabilizing microenvironment for the enzyme.
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Citations
Cited by
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Mohan, D., Pittman, C. U., & Steele, P. H. (2006) · Energy & Fuels · doi:10.1021/ef0502397 · Cited by 5,663
Ionic liquid processing of cellulose
Wang, H., Gurau, G., & Rogers, R. D. (2012) · Chemical Society Reviews · doi:10.1039/c2cs15311d · Cited by 1,369
Self-citationDissolution of cellulose with ionic liquids and its application: a mini-review
Zhu, S., Wu, Y., Chen, Q., Yu, Z., Wang, C., Jin, S., Ding, Y., & Wu, G. (2006) · Green Chemistry · doi:10.1039/b601395c · Cited by 1,260
Cellulose dissolution with polar ionic liquids under mild conditions: required factors for anions
Fukaya, Y., Hayashi, K., Wada, M., & Ohno, H. (2008) · Green Chem. · doi:10.1039/b713289a · Cited by 775
Rheological Properties of Cellulose/Ionic Liquid Solutions: From Dilute to Concentrated States
Gericke, M., Schlufter, K., Liebert, T., Heinze, T., & Budtova, T. (2009) · Biomacromolecules · doi:10.1021/bm801430x · Cited by 276
Cellulose Solvents – Remarkable History, Bright Future
Liebert, T. (2010) · ACS Symposium Series · doi:10.1021/bk-2010-1033.ch001 · Cited by 250
Aravamudhan, A., Ramos, D. M., Nada, A. A., & Kumbar, S. G. (2014) · Natural and Synthetic Biomedical Polymers · doi:10.1016/b978-0-12-396983-5.00004-1 · Cited by 238
Viscosity of Cellulose−Imidazolium-Based Ionic Liquid Solutions
Sescousse, R., Le, K. A., Ries, M. E., & Budtova, T. (2010) · The Journal of Physical Chemistry B · doi:10.1021/jp1024203 · Cited by 178
Sathitsuksanoh, N., Zhu, Z., & Zhang, Y.-H. P. (2012) · Cellulose · doi:10.1007/s10570-012-9719-z · Cited by 63
Ionic liquids in enzymatic catalysis and biochemical methods of analysis: Capabilities and prospects
Muginova, S. V., Galimova, A. Z., Polyakov, A. E., & Shekhovtsova, T. N. (2010) · Journal of Analytical Chemistry · doi:10.1134/s1061934810040027 · Cited by 36
Metadata
- Authors
- Turner, M. B., Spear, S. K., Holbrey, J. D., & Rogers, R. D.
- Venue
- Biomacromolecules
- Publisher
- American Chemical Society (ACS)
- Published
- 2004-06-22
- Volume
- 5
- Issue
- 4
- Pages
- 1379-1384
- ISSN
- 1525-7797 (ISSN-L)
- 1526-4602
- OpenAlex
- W2139774834
- Cited by
- 344
- References
- 0
- FWCI
- 6.86
- Type
- journal article
- Language
- en
- Open access
- closed
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