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Organic Photocatalysts for the Oxidation of Pollutants and Model Compounds

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Marin, M. Luisa, Santos-Juanes, Lucas, Arques, Antonio, Amat, Ana M., Miranda, Miguel A.·2012·Chemical Reviews

DOI 10.1021/cr2000543

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Abstract

The use of organic photocatalysts for the oxidation of pollutants and model compounds, with special emphasis on the involved concepts and mechanistic aspects, is reviewed. Photoinduced electron transfer involving the singlet excited state of phthalocyanines has been postulated in the photodegradation of phenols. The reactivity of OH - radical with different pollutants has been quantitatively determined by competition experiments, looking at the decrease of the typical transient absorption of the stilbene adduct at 390 nm. As regards heterogeneous media, after excitation at 355 nm of phthalocyanines immobilized in zeolites, the characteristic singlet oxygen luminiscence is monitored at 1270 nm. TPP has been included within extralarge pore zeolitic aluminosilicates, such as MCM-41. These materials provide an adequate balance between moderate cage effect and facilitation of molecular traffic through the mesopores.

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See all 426

Authors: Marin, M. L., Santos-Juanes, L., Arques, A., Amat, A. M., & Miranda, M. A.
Venue: Chemical Reviews
Publisher: American Chemical Society (ACS)
Published: 2011-10-31
Volume: 112
Issue: 3
Pages: 1710-1750
ISSN: 0009-2665 (ISSN-L)
1520-6890
DOI: 10.1021/cr2000543
OpenAlex: W2312778331
Cited by: 426
References: 124
FWCI: 1.44
Type: journal article
Language: en
Open access: green

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Organic Photocatalysts for the Oxidation of Pollutants and Model Compounds

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