Adsorption-Partitioning Uptake of Nine Low-Polarity Organic Chemicals on a Natural Sorbent
Abstract
Sorption of comparatively nonpolar organic chemicals by natural solids not only can be predominated by partitioning with organic matter but also can reflect a substantial contribution from adsorption at low relative concentration. Sorption of nine polycyclic aromatic hydrocarbons (PAHs) and chlorinated benzenes (CBs) was investigated on a subsurface aquitard through batch study, with results interpreted by a composite adsorption-partitioning model. For both PAHs and CBs, the low-concentration adsorption slope and the coefficient for partitioning each correlated well with K ow; however, PAHs consistently sorbed more strongly than CBs at given K ow . For all chemicals, adsorption contributions were only important at low relative concentration and could be successfully modeled by assuming either Langmuir-type or Polanyi-type isotherms. Isotherms for all liquid chemicals fell on a single isotherm when plotted on a Polanyi basis (adsorbed volume per mass of sorbent versus adsorption potential density), providing evidence that a pore-filling phenomenon is involved. Adsorbed volumes of solid chemicals were observed to be less than those of liquids at the same adsorption potential density, consistent with a reduction in packing efficiency and as previously reported for activated carbons. These results suggest that the adsorption contribution is from pore filling within microporous solids.
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The carbonized fraction is similar to the ''glassy'' fraction and the non-carbonized fraction is similar to the ''soft'' fraction.
“The carbonized fraction is similar to the ''glassy'' fraction (analogous to glassy polymers), and the non-carbonized fraction is similar to the ''soft'' fraction (analogous to rubbery polymers) (Xia and Ball 1999).”
From Biochar physicochemical properties: pyrolysis temperature and feedstock kind effects (2020) · cites this paper as Xia and Ball 1999
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- Authors
- Xia, G., & Ball, W. P.
- Affiliations
- Johns Hopkins University (US)
- ORCID
- Ball, William P.
- Venue
- Environmental Science & Technology
- Publisher
- American Chemical Society (ACS)
- Published
- 1998-12-05
- Volume
- 33
- Issue
- 2
- Pages
- 262-269
- ISSN
- 0013-936X (ISSN-L)
- 1520-5851
- OpenAlex
- W2024258880
- Cited by
- 262
- References
- 42
- Citations by year
- 2026: 2 · 2025: 5 · 2024: 1 · 2023: 5 · 2022: 4 · 2021: 5 · 2020: 11 · 2019: 2 · 2018: 6 · 2017: 6 · 2016: 6 · 2015: 4 · 2014: 17 · 2013: 11 · 2012: 11
- FWCI
- 11.80
- Type
- journal article
- Language
- en
- Open access
- closed
- Locations
- Environmental Science & Technology (publishedVersion)
- Topics
- Physical Sciences › Environmental Science › Water Science and Technology › Adsorption and biosorption for pollutant removal
- Physical Sciences › Environmental Science › Environmental Engineering › Groundwater flow and contamination studies
- Physical Sciences › Chemistry › Spectroscopy › Adsorption, diffusion, and thermodynamic properties of materials
- Keywords
- polycyclic aromatic hydrocarbons, chlorinated benzenes, natural adsorbents, aquitard, octanol-water partition coefficient, Langmuir isotherm, pore filling, microporous materials, sorption modeling, subsurface contaminant transport
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Registry, retraction, Cites and statistics results are computed, not judged, with one exception: a printed reference that no index lists is read once by a model before it counts as a citation error. Claims are extracted by a model and kept only when their quote appears verbatim in the text; each cited source is then checked, with a model’s help, for whether it says what the claim relies on. Those verdicts can be wrong — read the claim’s quote and the cited source before relying on one.
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