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Change of CO2Carrying Capacity of CaO in Isothermal Recarbonation−Decomposition Cycles
Abstract
The change of CO 2 carrying capacity of CaO sorbents prepared from different precursors has been studied using thermogravimetric analysis in a long series of isothermal recarbonation−decomposition cycles in the temperature range of 750−850 °C. The residual capacity of the CaO sorbents after a large number of cycles was found to depend on the precursor type, the experimental temperature, and the duration of the recarbonation stage. The residual capacities of the CaO derived from the powdered calcium carbonates were much higher than that of the CaO produced from the crystalline CaCO 3 . A simple tentative model has been suggested, according to which recarbonation−decomposition cycles result in formation of the interconnected CaO network that acts as a refractory support and determines sorption properties of the material. By using a new model, a simple synthesis procedure has been suggested that produces CaO sorbents with high residual CO 2 carrying capacities.
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Cites
Thermochemical Data of Pure Substances
Barin, I. (1995) · doi:10.1002/9783527619825 · Cited by 4,241
Cited by
CO2 capture by solid adsorbents and their applications: current status and new trends
Wang, Q., Luo, J., Zhong, Z., & Borgna, A. (2011) · Energy Environ. Sci. · doi:10.1039/c0ee00064g · Cited by 1,611
The calcium looping cycle for large-scale CO2 capture
Blamey, J., Anthony, E. J., Wang, J., & Fennell, P. S. (2010) · Progress in Energy and Combustion Science · doi:10.1016/j.pecs.2009.10.001 · Cited by 1,044
Review of recent advances in carbon dioxide separation and capture
Kenarsari, S. D., Yang, D., Jiang, G., Zhang, S., Wang, J., Russell, A. G., Wei, Q., & Fan, M. (2013) · RSC Advances · doi:10.1039/c3ra43965h · Cited by 784
Dean, C. C., Blamey, J., Florin, N. H., Al-Jeboori, M. J., & Fennell, P. S. (2011) · Chemical Engineering Research and Design · doi:10.1016/j.cherd.2010.10.013 · Cited by 375
Calcium looping sorbents for CO2 capture
Erans, M., Manovic, V., & Anthony, E. J. (2016) · Applied Energy · doi:10.1016/j.apenergy.2016.07.074 · Cited by 369
Metadata
- Authors
- Lysikov, A. I., Salanov, A. N., & Okunev, A. G.
- Venue
- Industrial & Engineering Chemistry Research
- Publisher
- American Chemical Society (ACS)
- Published
- 2007-05-15
- Volume
- 46
- Issue
- 13
- Pages
- 4633-4638
- ISSN
- 0888-5885 (ISSN-L)
- 1520-5045
- OpenAlex
- W2141510090
- Cited by
- 278
- References
- 1
- FWCI
- 38.37
- Type
- journal article
- Language
- en
- Open access
- closed
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