The DOI matches its Crossref record; 19 of the 19 references it cites were found in a registry or an index.
Assembly of Metal−Organic Frameworks from Large Organic and Inorganic Secondary Building Units: New Examples and Simplifying Principles for Complex Structures
Abstract
The secondary building unit (SBU) has been identified as a useful tool in the analysis of complex metal-organic frameworks (MOFs). We illustrate its applicability to rationalizing MOF crystal structures by analysis of nine new MOFs which have been characterized by single-crystal X-ray diffraction. Tetrahedral SBUs in Zn(ADC)(2).(HTEA)(2) (MOF-31), Cd(ATC).[Cd(H(2)O)(6)](H2O)(5) (MOF-32), and Zn(2)(ATB)(H2O).(H2O)(3)(DMF)(3) (MOF-33) are linked into diamond networks, while those of Ni(2)(ATC)(H(2)O)(4).(H2O)(4) (MOF-34) have the structure of the Al network in SrAl(2). Frameworks constructed from less symmetric tetrahedral SBUs have the Ga network of CaGa(2)O(4) as illustrated by Zn(2)(ATC).(C(2)H(5)OH)(2)(H2O)(2) (MOF-35) structure. Squares and tetrahedral SBUs in Zn(2)(MTB)(H2O)(2).(DMF)(6)(H2O)(5) (MOF-36) are linked into the PtS network, which is the simplest structure type known for the assembly of these shapes. The octahedral SBUs found in Zn(2)(NDC)(3).[(HTEA)(DEF)(ClBz)](2) (MOF-37) form the most common structure for linking octahedral shapes, namely, the boron network in CaB(6). New structure types for linking triangular and trigonal prismatic SBUs are found in Zn(3)O(BTC)(2).(HTEA)(2) (MOF-38) and Zn(3)O(HBTB)(2)(H2O).(DMF)(0.5)(H2O)(3) (MOF-39). The synthesis, crystal structure, and structure analysis using the SBU approach are presented for each MOF.
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Evaluating topologically diverse metal–organic frameworks for cryo-adsorbed hydrogen storage
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Metadata
- Authors
- Kim, J., Chen, B., Reineke, T. M., Li, H., Eddaoudi, M., Moler, D. B., O'Keeffe, M., & Yaghi, O. M.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2001-08-01
- Volume
- 123
- Issue
- 34
- Pages
- 8239-8247
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2014054292
- Cited by
- 832
- References
- 19
- FWCI
- 19.72
- Type
- journal article
- Language
- en
- Open access
- closed
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- Kim, J., Chen, B., Reineke, T. M., Li, H., Eddaoudi, M., Moler, D. B., O'Keeffe, M., & Yaghi, O. M. (2001). Assembly of Metal−Organic Frameworks from Large Organic and Inorganic Secondary Building Units: New Examples and Simplifying Principles for Complex Structures. Journal of the American Chemical Society. https://doi.org/10.1021/ja010825o
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