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Designing PbSe Nanowires and Nanorings through Oriented Attachment of Nanoparticles
Abstract
Single-crystal PbSe nanowires are synthesized in solution through oriented attachment of nanocrystal building blocks. Reaction temperatures of 190-250 degrees C and multicomponent surfactant mixtures result in a nearly defect-free crystal lattice and high uniformity of nanowire diameter along the entire length. The wires' dimensions are tuned by tailoring reaction conditions in a range from approximately 4 to approximately 20 nm in diameter with wire lengths up to approximately 30 microm. PbSe nanocrystals bind to each other on either {100}, {110}, or {111} faces, depending on the surfactant molecules present in the reaction solution. While PbSe nanocrystals have the centrosymmetric rocksalt lattice, they can lack central symmetry due to a noncentrosymmetric arrangement of Pb- and Se-terminated {111} facets and possess dipole driving one-dimensional oriented attachment of nanocrystals to form nanowires. In addition to straight nanowires, zigzag, helical, branched, and tapered nanowires as well as single-crystal nanorings can be controllably prepared in one-pot reactions by careful adjustment of the reaction conditions.
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Metadata
- Authors
- Cho, K.-S., Talapin, D. V., Gaschler, W., & Murray, C. B.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2005-04-23
- Volume
- 127
- Issue
- 19
- Pages
- 7140-7147
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2074188625
- Cited by
- 1,215
- References
- 1
- FWCI
- 43.53
- Type
- journal article
- Language
- en
- Open access
- closed
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