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A Mechanism for Non-stoichiometry in the Lithium Amide/Lithium Imide Hydrogen Storage Reaction
Abstract
We demonstrate, through structural refinement from synchrotron X-ray diffraction data, that the mechanism of the transformation between lithium amide and lithium imide during hydrogen cycling in the important Li-N-H hydrogen storage system is a bulk reversible reaction that occurs in a non-stoichiometric manner within the cubic anti-fluorite-like Li-N-H structure.
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Citations
Cited by
Complex Hydrides for Hydrogen Storage
Orimo, S.-I., Nakamori, Y., Eliseo, J. R., Züttel, A., & Jensen, C. M. (2007) · Chemical Reviews · doi:10.1021/cr0501846 · Cited by 2,318
Hydrogen Storage Materials for Mobile and Stationary Applications: Current State of the Art
Lai, Q., Paskevicius, M., Sheppard, D. A., Buckley, C. E., Thornton, A. W., Hill, M. R., Gu, Q., Mao, J., Huang, Z., Liu, H. K., et al. (2015) · ChemSusChem · doi:10.1002/cssc.201500231 · Cited by 414
Production of ammonia via a chemical looping process based on metal imides as nitrogen carriers
Gao, W., Guo, J., Wang, P., Wang, Q., Chang, F., Pei, Q., Zhang, W., Liu, L., & Chen, P. (2018) · Nature Energy · doi:10.1038/s41560-018-0268-z · Cited by 346
Shadike, Z., Lee, H., Borodin, O., Cao, X., Fan, X., Wang, X., Lin, R., Bak, S.-M., Ghose, S., Xu, K., et al. (2021) · Nature Nanotechnology · doi:10.1038/s41565-020-00845-5 · Cited by 320
Complex hydrides for energy storage, conversion, and utilization
He, T., Cao, H., & Chen, P. (2019) · Advanced Materials · doi:10.1002/adma.201902757 · Cited by 256
Metadata
- Authors
- David, W. I. F., Jones, M. O., Gregory, D. H., Jewell, C. M., Johnson, S. R., Walton, A., & Edwards, P. P.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2007-01-23
- Volume
- 129
- Issue
- 6
- Pages
- 1594-1601
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2043906247
- Cited by
- 256
- References
- 0
- FWCI
- 10.24
- Type
- journal article
- Language
- en
- Open access
- closed
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- David, W. I. F., Jones, M. O., Gregory, D. H., Jewell, C. M., Johnson, S. R., Walton, A., & Edwards, P. P. (2007). A Mechanism for Non-stoichiometry in the Lithium Amide/Lithium Imide Hydrogen Storage Reaction. Journal of the American Chemical Society. https://doi.org/10.1021/ja066016s
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