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Metal-Organic Framework from an Anthracene Derivative Containing Nanoscopic Cages Exhibiting High Methane Uptake
Abstract
A microporous metal-organic framework, PCN-14, based on an anthracene derivative, 5,5'-(9,10-anthracenediyl)di-isophthalate (H4adip), was synthesized under solvothermal reaction conditions. X-ray single crystal analysis revealed that PCN-14 consists of nanoscopic cages suitable for gas storage. N2-adsorption studies of PCN-14 at 77 K reveal a Langmuir surface area of 2176 m2/g and a pore volume of 0.87 cm3/g. Methane adsorption studies at 290 K and 35 bar show that PCN-14 exhibits an absolute methane-adsorption capacity of 230 v/v, 28% higher than the DOE target (180 v/v) for methane storage.
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Cited by
Large-scale screening of hypothetical metal–organic frameworks
Wilmer, C. E., Leaf, M., Lee, C. Y., Farha, O. K., Hauser, B. G., Hupp, J. T., & Snurr, R. Q. (2012) · Nature Chemistry · doi:10.1038/nchem.1192 · Cited by 1,439
Methane Storage in Metal–Organic Frameworks: Current Records, Surprise Findings, and Challenges
Peng, Y., Krungleviciute, V., Eryazici, I., Hupp, J. T., Farha, O. K., & Yildirim, T. (2013) · Journal of the American Chemical Society · doi:10.1021/ja4045289 · Cited by 1,018
Kökçam-Demir, Ü., Goldman, A., Esrafili, L., Gharib, M., Morsali, A., Weingart, O., & Janiak, C. (2020) · Chemical Society Reviews · doi:10.1039/c9cs00609e · Cited by 895
Carbide‐Derived Carbons – From Porous Networks to Nanotubes and Graphene
Presser, V., Heon, M., & Gogotsi, Y. (2011) · Advanced Functional Materials · doi:10.1002/adfm.201002094 · Cited by 678
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Colón, Y. J., & Snurr, R. Q. (2014) · Chem. Soc. Rev. · doi:10.1039/c4cs00070f · Cited by 470
Metadata
- Authors
- Ma, S., Sun, D., Simmons, J. M., Collier, C. D., Yuan, D., & Zhou, H.-C.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2007-12-29
- Volume
- 130
- Issue
- 3
- Pages
- 1012-1016
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2084852727
- Cited by
- 876
- References
- 0
- FWCI
- 44.23
- Type
- journal article
- Language
- en
- Open access
- closed
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- Ma, S., Sun, D., Simmons, J. M., Collier, C. D., Yuan, D., & Zhou, H.-C. (2008). Metal-Organic Framework from an Anthracene Derivative Containing Nanoscopic Cages Exhibiting High Methane Uptake. Journal of the American Chemical Society. https://doi.org/10.1021/ja0771639
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