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Metal-Organic Framework from an Anthracene Derivative Containing Nanoscopic Cages Exhibiting High Methane Uptake
Abstract
A microporous metal-organic framework, PCN-14, based on an anthracene derivative, 5,5'-(9,10-anthracenediyl)di-isophthalate (H4adip), was synthesized under solvothermal reaction conditions. X-ray single crystal analysis revealed that PCN-14 consists of nanoscopic cages suitable for gas storage. N2-adsorption studies of PCN-14 at 77 K reveal a Langmuir surface area of 2176 m2/g and a pore volume of 0.87 cm3/g. Methane adsorption studies at 290 K and 35 bar show that PCN-14 exhibits an absolute methane-adsorption capacity of 230 v/v, 28% higher than the DOE target (180 v/v) for methane storage.
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Metadata
- Authors
- Ma, S., Sun, D., Simmons, J. M., Collier, C. D., Yuan, D., & Zhou, H.-C.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2007-12-29
- Volume
- 130
- Issue
- 3
- Pages
- 1012-1016
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2084852727
- Cited by
- 876
- References
- 0
- FWCI
- 44.23
- Type
- journal article
- Language
- en
- Open access
- closed
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