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Structural Evolution of Zeolitic Imidazolate Framework-8
Abstract
We report the structural evolution of zeolitic imidazolate framework-8 (ZIF-8) as a function of time at room temperature. We have identified the different stages of ZIF-8 formation (nucleation, crystallization, growth, and stationary periods) and elucidated its kinetics of transformation. We hypothesize that the observed semicrystalline-to-crystalline transformation may take place via solution- and solid-mediated mechanisms, as suggested by the observed phase transformation evolution and Avrami's kinetics, respectively. A fundamental understanding of ZIF-8 structural evolution as demonstrated in this study should facilitate the preparation of functional metal-organic framework phases with controlled crystal size and extent of crystallinity.
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Cited by
Cravillon, J., Nayuk, R., Springer, S., Feldhoff, A., Huber, K., & Wiebcke, M. (2011) · Chemistry of Materials · doi:10.1021/cm103571y · Cited by 916
Zhan, W.-W., Kuang, Q., Zhou, J.-Z., Kong, X.-J., Xie, Z.-X., & Zheng, L.-S. (2013) · Journal of the American Chemical Society · doi:10.1021/ja311085e · Cited by 803
Multifunctional metal–organic framework heterostructures for enhanced cancer therapy
Liu, J., Huang, J., Zhang, L., & Lei, J. (2021) · Chemical Society Reviews · doi:10.1039/d0cs00178c · Cited by 285
Gene Delivery Technologies with Applications in Microalgal Genetic Engineering
Gutiérrez, S., & Lauersen, K. J. (2021) · Biology · doi:10.3390/biology10040265 · Cited by 68
Li, Q., Xiao, X., Yan, T., Song, D., Li, L., Chen, Z., Zhong, Y., Deng, W., Liu, X., Song, Y., et al. (2024) · ACS Applied Materials & Interfaces · doi:10.1021/acsami.4c15715 · Cited by 20
Metadata
- Authors
- Venna, S. R., Jasinski, J. B., & Carreon, M. A.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2010-12-06
- Volume
- 132
- Issue
- 51
- Pages
- 18030-18033
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W1983228317
- Cited by
- 857
- References
- 0
- FWCI
- 10.68
- Type
- journal article
- Language
- en
- Open access
- closed
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- Venna, S. R., Jasinski, J. B., & Carreon, M. A. (2010). Structural Evolution of Zeolitic Imidazolate Framework-8. Journal of the American Chemical Society. https://doi.org/10.1021/ja109268m
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