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Tetravalent Metal Complexes as a New Family of Catalysts for Copolymerization of Epoxides with Carbon Dioxide
Abstract
New tetravalent metal complexes with a trianionic [ONNO]-tetradentate ligand and an ancillary chloride ligand were synthesized as catalysts for the copolymerization of epoxides with carbon dioxide (CO(2)). All of the titanium, zirconium, germanium, and tin complexes were found to copolymerize epoxides with CO(2). In particular, the copolymerization of propylene oxide with CO(2) gave the almost-completely alternating copolymers by using titanium or germanium complexes. These results are the first example of the copolymerization using tetravalent metal complexes as a main component of catalysts.
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Darensbourg, D. J. (2007) · Chemical Reviews · doi:10.1021/cr068363q · Cited by 1,593
Cited by
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Recent progress in catalytic conversions of carbon dioxide
Maeda, C., Miyazaki, Y., & Ema, T. (2014) · Catalysis Science & Technology · doi:10.1039/c3cy00993a · Cited by 517
Controlled Polymerization of Next-Generation Renewable Monomers and Beyond
Yao, K., & Tang, C. (2013) · Macromolecules · doi:10.1021/ma3019574 · Cited by 485
Ema, T., Miyazaki, Y., Shimonishi, J., Maeda, C., & Hasegawa, J.-Y. (2014) · Journal of the American Chemical Society · doi:10.1021/ja507665a · Cited by 473
Park, J. H., Jeon, J. Y., Lee, J. J., Jang, Y., Varghese, J. K., & Lee, B. Y. (2013) · Macromolecules · doi:10.1021/ma400360w · Cited by 158
Metadata
- Authors
- Nakano, K., Kobayashi, K., & Nozaki, K.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2011-06-23
- Volume
- 133
- Issue
- 28
- Pages
- 10720-10723
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2152762735
- Cited by
- 182
- References
- 1
- FWCI
- 6.97
- Type
- journal article
- Language
- en
- Open access
- closed
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