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Oxygen Radical Functionalization of Boron Nitride Nanosheets
Open accessAbstract
The covalent chemical functionalization of exfoliated hexagonal boron-nitride nanosheets (BNNSs) is achieved by the solution-phase oxygen radical functionalization of boron atoms in the h-BN lattice. This involves a two-step procedure to initially covalently graft alkoxy groups to boron atoms and the subsequent hydrolytic defunctionalization of the groups to yield hydroxyl-functionalized BNNSs (OH-BNNSs). Characterization of the functionalized-BNNSs using HR-TEM, Raman, UV-vis, FTIR, NMR, and TGA was performed to investigate both the structure of the BNNSs and the covalent functionalization methodology. OH-BNNSs were used to prepare polymer nanocomposites and their mechanical properties analyzed. The influence of the functional groups grafted to the surface of the BNNSs is investigated by demonstrating the impact on mechanical properties of both noncovalent and covalent bonding at the interface between the nanofiller and polymer matrixes.
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Graphene-based composite materials
Stankovich, S., Dikin, D. A., Dommett, G. H. B., Kohlhaas, K. M., Zimney, E. J., Stach, E. A., Piner, R. D., Nguyen, S. T., & Ruoff, R. S. (2006) · Nature · doi:10.1038/nature04969 · Cited by 12,922
Two-dimensional atomic crystals
Novoselov, K. S., Jiang, D., Schedin, F., Booth, T. J., Khotkevich, V. V., Morozov, S. V., & Geim, A. K. (2005) · Proceedings of the National Academy of Sciences · doi:10.1073/pnas.0502848102 · Cited by 11,788
Cited by
Highly Water-Soluble, Porous, and Biocompatible Boron Nitrides for Anticancer Drug Delivery
Weng, Q., Wang, B., Wang, X., Hanagata, N., Li, X., Liu, D., Wang, X., Jiang, X., Bando, Y., & Golberg, D. (2014) · ACS Nano · doi:10.1021/nn5014808 · Cited by 455
Functionalization of Nanomaterials: Synthesis and Characterization
Rizvi, M., Gerengi, H., & Gupta, P. (2022) · ACS Symposium Series · doi:10.1021/bk-2022-1418.ch001 · Cited by 55
Metadata
- Authors
- Sainsbury, T., Satti, A., May, P., Wang, Z., McGovern, I., Gun’ko, Y. K., & Coleman, J.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2012-11-05
- Volume
- 134
- Issue
- 45
- Pages
- 18758-18771
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2048585881
- Cited by
- 575
- References
- 2
- FWCI
- 6.52
- Type
- journal article
- Language
- en
- Open access
- green
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- Sainsbury, T., Satti, A., May, P., Wang, Z., McGovern, I., Gun’ko, Y. K., & Coleman, J. (2012). Oxygen Radical Functionalization of Boron Nitride Nanosheets. Journal of the American Chemical Society. https://doi.org/10.1021/ja3080665
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