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Electric Field-Induced Assembly of Monodisperse Polyhedral Metal–Organic Framework Crystals
Abstract
Monodisperse polyhedral metal-organic framework (MOF) particles up to 5 μm in size, large enough to enable in situ optical imaging of particle orientation, were synthesized by the strategy of simultaneous addition of two capping ligands with different binding strength during crystallization. Upon dispersing them in ethylene glycol and applying AC electric field, the particles facets link to form linear chains. We observe well-regulated crystal orientation not only for rhombic dodecahedra all of whose facets are equivalent, but also for truncated cubes with nondegenerate facets. After removing the electric field, chains disassemble if their facets contain even modest curvature, but remain intact if their facets are planar. This assembly strategy offers a general route to fabricate oriented polyhedral crystal arrays of potential interest for new applications and functions.
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Cites
Metal-organic framework materials as catalysts
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Boles, M. A., Engel, M., & Talapin, D. V. (2016) · Chemical Reviews · doi:10.1021/acs.chemrev.6b00196 · Cited by 2,051
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The surface chemistry of metal–organic frameworks
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Tackling orientation of metal-organic frameworks (MOFs): The quest to enhance MOF performance
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MOF based engineered materials in water remediation: Recent trends
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Controllable Synthesis of Metal-Organic Frameworks and Their Hierarchical Assemblies
Feng, L., Wang, K.-Y., Powell, J., & Zhou, H.-C. (2019) · Matter · doi:10.1016/j.matt.2019.08.022 · Cited by 266
Self-assembly of anisotropic nanoparticles into functional superstructures
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Metadata
- Authors
- Yanai, N., Sindoro, M., Yan, J., & Granick, S.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2012-12-20
- Volume
- 135
- Issue
- 1
- Pages
- 34-37
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2329180172
- Cited by
- 188
- References
- 2
- FWCI
- 6.29
- Type
- journal article
- Language
- en
- Open access
- closed
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