The DOI matches its Crossref record; 34 of the 34 references it cites were found in a registry or an index.
Tunable Rare-Earth fcu-MOFs: A Platform for Systematic Enhancement of CO2 Adsorption Energetics and Uptake
Abstract
A series of fcu-MOFs based on rare-earth (RE) metals and linear fluorinated/nonfluorinated, homo/heterofunctional ligands were targeted and synthesized. This particular fcu-MOF platform was selected because of its unique structural characteristics combined with the ability/potential to dictate and regulate its chemical properties (e.g., tuning of the electron-rich RE metal ions and high localized charge density, a property arising from the proximal positioning of polarizing tetrazolate moieties and fluoro-groups that decorate the exposed inner surfaces of the confined conical cavities). These features permitted a systematic gas sorption study to evaluate/elucidate the effects of distinctive parameters on CO2-MOF sorption energetics. Our study supports the importance of the synergistic effect of exposed open metal sites and proximal highly localized charge density toward materials with enhanced CO2 sorption energetics.
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Metadata
- Authors
- Xue, D.-X., Cairns, A. J., Belmabkhout, Y., Wojtas, L., Liu, Y., Alkordi, M. H., & Eddaoudi, M.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2013-05-07
- Volume
- 135
- Issue
- 20
- Pages
- 7660-7667
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2318655974
- Cited by
- 531
- References
- 34
- FWCI
- 26.24
- Type
- journal article
- Language
- en
- Open access
- closed
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- Xue, D.-X., Cairns, A. J., Belmabkhout, Y., Wojtas, L., Liu, Y., Alkordi, M. H., & Eddaoudi, M. (2013). Tunable Rare-Earth fcu-MOFs: A Platform for Systematic Enhancement of CO2 Adsorption Energetics and Uptake. Journal of the American Chemical Society. https://doi.org/10.1021/ja401429x
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