The DOI matches its Crossref record; 2 of the 2 references it cites were found in a registry or an index.
Core-Shell Nanostructured “Black” Rutile Titania as Excellent Catalyst for Hydrogen Production Enhanced by Sulfur Doping
Abstract
Modification of rutile titanium dioxide (TiO2) for hydrogen generation and water cleaning is a grand challenge due to the chemical inertness of rutile, while such inertness is a desired merit for its stability in photoelectrochemical applications. Herein, we report an innovative two-step method to prepare a core-shell nanostructured S-doped rutile TiO2 (R'-TiO2-S). This modified black rutile TiO2 sample exhibits remarkably enhanced absorption in visible and near-infrared regions and efficient charge separation and transport. As a result, the unique sulfide surface (TiO(2-x):S) boosts the photocatalytic water cleaning and water splitting with a steady solar hydrogen production rate of 0.258 mmol h(-1) g(-1). The black titania is also an excellent photoelectrochemical electrode exhibiting a high solar-to-hydrogen conversion efficiency of 1.67%. The sulfided surface shell is proved to be an effective strategy for enhancing solar light absorption and photoelectric conversion.
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Cites
Environmental applications of semiconductor photocatalysis
Hoffmann, M. R., Martin, S. T., Choi, W., & Bahnemann, D. W. (1995) · Chemical Reviews · doi:10.1021/cr00033a004 · Cited by 18,495
Photocatalysis on TiO2 Surfaces: Principles, Mechanisms, and Selected Results
Linsebigler, A. L., Lu, G., & Yates, J. T. (1995) · Chemical Reviews · doi:10.1021/cr00035a013 · Cited by 11,575
Cited by
Yang, W., Prabhakar, R. R., Tan, J., Tilley, S. D., & Moon, J. (2019) · Chemical Society Reviews · doi:10.1039/c8cs00997j · Cited by 787
Constructing Black Titania with Unique Nanocage Structure for Solar Desalination
Zhu, G., Xu, J., Zhao, W., & Huang, F. (2016) · ACS Applied Materials & Interfaces · doi:10.1021/acsami.6b11466 · Cited by 357
Self-citationAdvanced Catalysts for Photoelectrochemical Water Splitting
Marwat, M. A., Humayun, M., Afridi, M. W., Zhang, H., Abdul Karim, M. R., Ashtar, M., Usman, M., Waqar, S., Ullah, H., Wang, C., et al. (2021) · ACS Applied Energy Materials · doi:10.1021/acsaem.1c02548 · Cited by 191
Metadata
- Authors
- Yang, C., Wang, Z., Lin, T., Yin, H., Lü, X., Wan, D., Xu, T., Zheng, C., Lin, J., Huang, F., Xie, X., & Jiang, M.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2013-11-14
- Volume
- 135
- Issue
- 47
- Pages
- 17831-17838
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2084409156
- Cited by
- 474
- References
- 2
- FWCI
- 12.98
- Type
- journal article
- Language
- en
- Open access
- closed
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- Yang, C., Wang, Z., Lin, T., Yin, H., Lü, X., Wan, D., Xu, T., Zheng, C., Lin, J., Huang, F., Xie, X., & Jiang, M. (2013). Core-Shell Nanostructured “Black” Rutile Titania as Excellent Catalyst for Hydrogen Production Enhanced by Sulfur Doping. Journal of the American Chemical Society. https://doi.org/10.1021/ja4076748
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