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Robust Cuprous Phenanthroline Sensitizer for Solar Hydrogen Photocatalysis
Open accessAbstract
The Cu(I) metal-to-ligand charge-transfer complex, [Cu(dsbtmp)2](+) (dsbtmp = 2,9-di(sec-butyl)-3,4,7,8-tetramethyl-1,10-phenanthroline), exhibits outstanding stability as a visible-light-absorbing photosensitizer in hydrogen-evolving homogeneous photocatalysis. In concert with the Co(dmgH)2(py)Cl water reduction catalyst and N,N-dimethyl-p-toluidine sacrificial donor in 1:1 H2O:CH3CN, this Cu(I) sensitizer remains active even after 5 days of visible-light-pumped (λex = 452 ± 10 nm) hydrogen evolution catalysis. Deuteration studies illustrate that the hydrogen produced from this composition does indeed originate from aqueous protons.
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Prier, C. K., Rankic, D. A., & MacMillan, D. W. C. (2013) · Chemical Reviews · doi:10.1021/cr300503r · Cited by 9,590
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Sacrificial electron donor reagents for solar fuel production
Pellegrin, Y., & Odobel, F. (2016) · Comptes Rendus. Chimie · doi:10.1016/j.crci.2015.11.026 · Cited by 561
Metal-complex chromophores for solar hydrogen generation
Yuan, Y.-J., Yu, Z.-T., Chen, D.-Q., & Zou, Z.-G. (2017) · Chemical Society Reviews · doi:10.1039/c6cs00436a · Cited by 423
Metadata
- Authors
- Khnayzer, R. S., McCusker, C. E., Olaiya, B. S., & Castellano, F. N.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2013-09-17
- Volume
- 135
- Issue
- 38
- Pages
- 14068-14070
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2318077607
- Cited by
- 167
- References
- 1
- FWCI
- 5.77
- Type
- journal article
- Language
- en
- Open access
- hybrid
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- Khnayzer, R. S., McCusker, C. E., Olaiya, B. S., & Castellano, F. N. (2013). Robust Cuprous Phenanthroline Sensitizer for Solar Hydrogen Photocatalysis. Journal of the American Chemical Society. https://doi.org/10.1021/ja407816f
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