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Bicontinuous Zeolitic Imidazolate Framework ZIF-8@GO Membrane with Enhanced Hydrogen Selectivity
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Through layer-by-layer (LBL) deposition of a graphene oxide (GO) suspension on a semicontinuous ZIF-8 layer, we have developed a novel bicontinuous ZIF-8@GO membrane. Since only the gaps between the ZIF-8 crystals are sealed by the GO layer due to capillary forces and covalent bonds, the gas molecules can only permeate through the ZIF-8 micropore system (0.34 nm). Therefore, the ZIF-8@GO membranes show high hydrogen selectivity. At 250 °C and 1 bar, the mixture separation factors of H2/CO2, H2/N2, H2/CH4, and H2/C3H8 are 14.9, 90.5, 139.1, and 3816.6, with H2 permeances of about 1.3 × 10(-7) mol·m(-2)·s(-1)·Pa(-1), which is promising for hydrogen separation and purification by molecular sieving.
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Metadata
- Authors
- Huang, A., Liu, Q., Wang, N., Zhu, Y., & Caro, J.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2014-10-10
- Volume
- 136
- Issue
- 42
- Pages
- 14686-14689
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2313827370
- Cited by
- 346
- References
- 40
- FWCI
- 30.00
- Type
- journal article
- Language
- en
- Open access
- green
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