The DOI matches its Crossref record; 1 of the 1 references it cites were found in a registry or an index.
Synthetic Control of the Pore Dimension and Surface Area in Conjugated Microporous Polymer and Copolymer Networks
Abstract
A series of rigid microporous poly(aryleneethynylene) (PAE) networks was synthesized by Sonogashira-Hagihara coupling chemistry. PAEs with apparent Brunauer-Emmet-Teller surface areas of more than 1000 m(2)/g were produced. The materials were found to have very good chemical and thermal stability and retention of microporosity under a variety of conditions. It was shown that physical properties such as micropore size, surface area, and hydrogen uptake could be controlled in a "quantized" fashion by varying the monomer strut length, as for metal-organic and covalent organic frameworks, even though the networks were amorphous in nature. For the first time, it was demonstrated that these properties can also be fine-tuned in a continuous manner via statistical copolymerization of monomer struts with differing lengths. This provides an unprecedented degree of direct synthetic control over micropore properties in an organic network.
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Cites
Sing, K. S. W. (1985) · Pure and Applied Chemistry · doi:10.1351/pac198557040603 · Cited by 24,485
Cited by
Wang, H., Zeng, Z., Xu, P., Li, L., Zeng, G., Xiao, R., Tang, Z., Huang, D., Tang, L., Lai, C., et al. (2019) · Chemical Society Reviews · doi:10.1039/c8cs00376a · Cited by 804
Yu, X., Tang, Z., Sun, D., Ouyang, L., & Zhu, M. (2017) · Progress in Materials Science · doi:10.1016/j.pmatsci.2017.03.001 · Cited by 716
Li, B., Gong, R., Wang, W., Huang, X., Zhang, W., Li, H., Hu, C., & Tan, B. (2011) · Macromolecules · doi:10.1021/ma200630s · Cited by 632
Superhydrophobic conjugated microporous polymers for separation and adsorption
Li, A., Sun, H.-X., Tan, D.-Z., Fan, W.-J., Wen, S.-H., Qing, X.-J., Li, G.-X., Li, S.-Y., & Deng, W.-Q. (2011) · Energy & Environmental Science · doi:10.1039/c1ee01092a · Cited by 601
Porous Polymers as Multifunctional Material Platforms toward Task‐Specific Applications
Wu, J., Xu, F., Li, S., Ma, P., Zhang, X., Liu, Q., Fu, R., & Wu, D. (2019) · Advanced Materials · doi:10.1002/adma.201802922 · Cited by 555
Metadata
- Authors
- Jiang, J.-X., Su, F., Trewin, A., Wood, C. D., Niu, H., Jones, J. T. A., Khimyak, Y. Z., & Cooper, A. I.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2008-05-24
- Volume
- 130
- Issue
- 24
- Pages
- 7710-7720
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2058236705
- Cited by
- 879
- References
- 1
- FWCI
- 18.69
- Type
- journal article
- Language
- en
- Open access
- closed
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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