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Influence of Size on the Rate of Mesoporous Electrodes for Lithium Batteries
Abstract
High power rechargeable lithium batteries are a key target for transport and load leveling, in order to mitigate CO(2) emissions. It has already been demonstrated that mesoporous lithium intercalation compounds (composed of particles containing nanometer diameter pores separated by walls of similar size) can deliver high rate (power) and high stability on cycling. Here we investigate how the critical dimensions of pore size and wall thickness control the rate of intercalation (electrode reaction). By using mesoporous beta-MnO(2), the influence of these mesodimensions on lithium intercalation via single and two-phase intercalation processes has been studied in the same material enabling direct comparison. Pore size and wall thickness both influence the rate of single and two-phase intercalation mechanisms, but the latter is more sensitive than the former.
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Cites
Sing, K. S. W. (1985) · Pure and Applied Chemistry · doi:10.1351/pac198557040603 · Cited by 24,485
Cited by
Nanostructured metal oxide-based materials as advanced anodes for lithium-ion batteries
Wu, H. B., Chen, J. S., Hng, H. H., & Wen (David) Lou, X. (2012) · Nanoscale · doi:10.1039/c2nr11966h · Cited by 1,082
Porous electrode materials for lithium-ion batteries–how to prepare them and what makes them special
Vu, A., Qian, Y., & Stein, A. (2012) · Advanced Energy Materials · doi:10.1002/aenm.201200320 · Cited by 719
Mesoporous materials and electrochemistry
Walcarius, A. (2013) · Chemical Society Reviews · doi:10.1039/c2cs35322a · Cited by 623
Conversion Reaction‐Based Oxide Nanomaterials for Lithium Ion Battery Anodes
Yu, S., Lee, S. H., Lee, D. J., Sung, Y., & Hyeon, T. (2016) · Small · doi:10.1002/smll.201502299 · Cited by 499
Jayaramulu, K., Dubal, D. P., Nagar, B., Ranc, V., Tomanec, O., Petr, M., Datta, K. K. R., Zboril, R., Gómez‐Romero, P., & Fischer, R. A. (2018) · Advanced Materials · doi:10.1002/adma.201705789 · Cited by 394
Metadata
- Authors
- Ren, Y., Armstrong, A. R., Jiao, F., & Bruce, P. G.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2009-12-29
- Volume
- 132
- Issue
- 3
- Pages
- 996-1004
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2010316566
- Cited by
- 282
- References
- 1
- FWCI
- 16.63
- Type
- journal article
- Language
- en
- Open access
- closed
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