The DOI matches its Crossref record; 40 of the 40 references it cites were found in a registry or an index.
Solid–Solution-Based Metal Alloy Phase for Highly Reversible Lithium Metal Anode
Abstract
Lithium metal batteries are vital devices for high-energy-density energy storage, but the Li metal anode is highly reactive with electrolyte and forms uncontrolled dendrite that can cause undesirable parasitic reactions and, thus, poor cycling stability and raise safety concerns. Despite remarkable progress to partially solve these issues, the Li metal still plates at the electrode/electrolyte interface where the parasitic reactions and dendrite formation invariably occur. Here, we demonstrate the inward-growth plating of Li atoms into a metal foil of thickness of tens of micrometers while avoiding surface deposition, which is driven by the reversible solid–solution-based alloy phase change. Lithiation of the solid–solution alloy phase allows the freshly generated Li atoms at the surface to sink into the metal foil, while the reversible alloy phase change is companied by the dealloying reaction during delithiation, which extracts Li atoms from inside of the metal foil. The yielded dendrite free Li anode produces an enhanced Coulombic efficiency of 99.5 ± 0.2% with a reversible capacity of 1660 mA h g –1 (3.3 mA h cm –2 ).
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Citations
Cites
Nonaqueous Liquid Electrolytes for Lithium-Based Rechargeable Batteries
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Reviving the lithium metal anode for high-energy batteries
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Toward Safe Lithium Metal Anode in Rechargeable Batteries: A Review
Cheng, X.-B., Zhang, R., Zhao, C.-Z., & Zhang, Q. (2017) · Chemical Reviews · doi:10.1021/acs.chemrev.7b00115 · Cited by 6,197
Pathways for practical high-energy long-cycling lithium metal batteries
Liu, J., Bao, Z., Cui, Y., Dufek, E. J., Goodenough, J. B., Khalifah, P., Li, Q., Liaw, B. Y., Liu, P., Manthiram, A., et al. (2019) · Nature Energy · doi:10.1038/s41560-019-0338-x · Cited by 3,412
Alloy Negative Electrodes for Li-Ion Batteries
Obrovac, M. N., & Chevrier, V. L. (2014) · Chemical Reviews · doi:10.1021/cr500207g · Cited by 2,175
Selective deposition and stable encapsulation of lithium through heterogeneous seeded growth
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Cited by
High‐Energy Lithium‐Ion Batteries: Recent Progress and a Promising Future in Applications
Xu, J., Cai, X., Cai, S., Shao, Y., Hu, C., Lu, S., & Ding, S. (2023) · ENERGY & ENVIRONMENTAL MATERIALS · doi:10.1002/eem2.12450 · Cited by 1,201
Electroless Formation of a Fluorinated Li/Na Hybrid Interphase for Robust Lithium Anodes
Wang, Y., Liu, F., Fan, G., Qiu, X., Liu, J., Yan, Z., Zhang, K., Cheng, F., & Chen, J. (2021) · Journal of the American Chemical Society · doi:10.1021/jacs.0c12051 · Cited by 283
Insights into the deposition chemistry of Li ions in nonaqueous electrolyte for stable Li anodes
Wang, Z., Sun, Z., Li, J., Shi, Y., Sun, C., An, B., Cheng, H.-M., & Li, F. (2021) · Chemical Society Reviews · doi:10.1039/d0cs01017k · Cited by 268
Self-citation
Metadata
- Authors
- Jin, S., Ye, Y., Niu, Y., Xu, Y., Jin, H., Wang, J., Sun, Z., Cao, A., Wu, X., Luo, Y., Ji, H., & Wan, L.-J.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2020-04-20
- Volume
- 142
- Issue
- 19
- Pages
- 8818-8826
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W3017151063
- Cited by
- 391
- References
- 40
- FWCI
- 15.02
- Type
- journal article
- Language
- en
- Open access
- closed
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- Jin, S., Ye, Y., Niu, Y., Xu, Y., Jin, H., Wang, J., Sun, Z., Cao, A., Wu, X., Luo, Y., Ji, H., & Wan, L.-J. (2020). Solid–Solution-Based Metal Alloy Phase for Highly Reversible Lithium Metal Anode. Journal of the American Chemical Society. https://doi.org/10.1021/jacs.0c01811
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