Determining the Interfacial Refractive Index via Ultrasensitive Plasmonic Sensors
Abstract
Plasmonic sensors are promising for ultrasensitive chemical and biological analysis. However, there are increasing experimental findings that cannot be well addressed by theoretical calculations, including the nonlinear dependence of the plasmonic peak wavelength on the refractive index (RI) and the ultrahigh sensitivity beyond the theoretical limit. The gap between experiments and theoretical calculations is that the bulk RI (BRI) used for calculation could be different from the interfacial RI (IRI) determining the electromagnetic response as a result of the interaction of molecules with the surface. But there is still no method to determine the IRI. Herein, we quantitatively determine the IRI by disentangling the surface RI (SRI) from the BRI. The obtained IRI can be directly applied in theoretical calculations to reliably reflect the experimental response and rigorously guide the design of plasmonic sensors. Moreover, it can be a fundamental dimensionless number to describe the light-matter interaction at the interface.
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Plasmonic nanoantennas serve as ultra-sensitive refractometry sensors to capture the refractive index of analytes by wavelength shifts.
“Thanks to the excellent field confinement at resonance wavelength, plasmonic nanoantennas (PNAs) also serve as an ultra-sensitive refractometry sensor to capture the refractive index of analytes by wavelength shifts (e.g., color change in visible light), which carries the information of physical properties of molecules44,45.”
From Wavelength-multiplexed hook nanoantennas for machine learning enabled mid-infrared spectroscopy (2022) · cites this paper as [45]
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- Authors
- Zhan, C., Liu, B.-W., Tian, Z.-Q., & Ren, B.
- Affiliations
- Xiamen University (CN)
- State Key Laboratory of Physical Chemistry of Solid Surfaces, College of Chemistry and Chemical Engineering, Collaborative Innovation Center of Chemistry for Energy Materials (iChEM), Xiamen University, Xiamen 361005, China
- Corresponding author
- Ren, Bin
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2020-06-08
- Volume
- 142
- Issue
- 25
- Pages
- 10905-10909
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W3033534775
- Cited by
- 56
- References
- 35
- Citations by year
- 2026: 3 · 2025: 11 · 2024: 5 · 2023: 10 · 2022: 13 · 2021: 11 · 2020: 3
- FWCI
- 2.90
- Type
- journal article
- Language
- en
- Open access
- closed
- Licence
- Locations
- Journal of the American Chemical Society (publishedVersion)
- PubMed (publishedVersion)
- Lanzhou University Institutional Repository (submittedVersion)
- Funders
- Ministry of Science and Technology of the People's Republic of China (2016YFA0200601)
- National Natural Science Foundation of China (21633005, 21711530704, 21790354, 21804061)
- Topics
- Physical Sciences › Engineering › Biomedical Engineering › Plasmonic and Surface Plasmon Research
- Physical Sciences › Materials Science › Electronic, Optical and Magnetic Materials › Gold and Silver Nanoparticles Synthesis and Applications
- Physical Sciences › Engineering › Electrical and Electronic Engineering › Advanced Fiber Optic Sensors
- Keywords
- plasmonic sensors, surface plasmon resonance, surface refractive index, sensor sensitivity
- MeSH terms
- Adsorption, Glycerol, Models, Chemical, Refractometry, Surface Plasmon Resonance
About these checks
Registry, retraction, Cites and statistics results are computed, not judged, with one exception: a printed reference that no index lists is read once by a model before it counts as a citation error. Claims are extracted by a model and kept only when their quote appears verbatim in the text; each cited source is then checked, with a model’s help, for whether it says what the claim relies on. Those verdicts can be wrong — read the claim’s quote and the cited source before relying on one.
Statistics and arithmetic are recomputed, not judged.
Confidence bands are shown only for fields calibrated on our annotated test set. None is calibrated yet, so no band is shown.
What counts as a claim ›How we measure confidence ›How we check this ›
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