The DOI matches its Crossref record; 1 of the 1 references it cites were found in a registry or an index.
Stable Covalent Organic Frameworks for Exceptional Mercury Removal from Aqueous Solutions
Abstract
The pre-designable porous structures found in covalent organic frameworks (COFs) render them attractive as a molecular platform for addressing environmental issues such as removal of toxic heavy metal ions from water. However, a rational structural design of COFs in this aspect has not been explored. Here we report the rational design of stable COFs for Hg(II) removal through elaborate structural design and control over skeleton, pore size, and pore walls. The resulting framework is stable under strong acid and base conditions, possesses high surface area, has large mesopores, and contains dense sulfide functional termini on the pore walls. These structural features work together in removing Hg(II) from water and achieve a benchmark system that combines capacity, efficiency, effectivity, applicability, selectivity, and reusability. These results suggest that COFs offer a powerful platform for tailor-made structural design to cope with various types of pollution.
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Cites
Fang, Q.-R., Yuan, D.-Q., Sculley, J., Li, J.-R., Han, Z.-B., & Zhou, H.-C. (2010) · Inorganic Chemistry · doi:10.1021/ic101935f · Cited by 309
Cited by
Liu, R., Tan, K. T., Gong, Y., Chen, Y., Li, Z., Xie, S., He, T., Lu, Z., Yang, H., & Jiang, D. (2021) · Chemical Society Reviews · doi:10.1039/d0cs00620c · Cited by 1,083
Self-citationA versatile MOF-based trap for heavy metal ion capture and dispersion
Peng, Y., Huang, H., Zhang, Y., Kang, C., Chen, S., Song, L., Liu, D., & Zhong, C. (2018) · Nature Communications · doi:10.1038/s41467-017-02600-2 · Cited by 804
Sun, Q., Aguila, B., Earl, L. D., Abney, C. W., Wojtas, L., Thallapally, P. K., & Ma, S. (2018) · Advanced Materials · doi:10.1002/adma.201705479 · Cited by 641
Porous Polymers as Multifunctional Material Platforms toward Task‐Specific Applications
Wu, J., Xu, F., Li, S., Ma, P., Zhang, X., Liu, Q., Fu, R., & Wu, D. (2019) · Advanced Materials · doi:10.1002/adma.201802922 · Cited by 555
Beuerle, F., & Gole, B. (2018) · Angewandte Chemie International Edition · doi:10.1002/anie.201710190 · Cited by 528
Metadata
- Authors
- Huang, N., Zhai, L., Xu, H., & Jiang, D.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2017-02-07
- Volume
- 139
- Issue
- 6
- Pages
- 2428-2434
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2580106504
- Cited by
- 680
- References
- 1
- FWCI
- 28.00
- Type
- journal article
- Language
- en
- Open access
- closed
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- Huang, N., Zhai, L., Xu, H., & Jiang, D. (2017). Stable Covalent Organic Frameworks for Exceptional Mercury Removal from Aqueous Solutions. Journal of the American Chemical Society. https://doi.org/10.1021/jacs.6b12328
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