The DOI matches its Crossref record; 14 of the 14 references it cites were found in a registry or an index.
Investigating the Influences of the Adsorbed Species on Catalytic Activity for Hydrogen Oxidation Reaction in Alkaline Electrolyte
Abstract
Abstract Catalysts for hydrogen oxidation reaction (HOR) in alkaline electrolyte are important for anion exchange membrane fuel cells. Understanding the role of OH– during the HOR catalytic process in alkaline electrolyte is essential to design highly active HOR catalysts. Here, we attempt to isolate the influence of OH– by using surface-controlled Pt based nanoparticles as the model catalysts. With a comparison of the HOR activity between PtNi nanoparticles and acid washed PtNi nanoparticles, which have almost the same hydrogen binding energies but much different OH binding energies, it was found that the HOR activity in alkaline electrolyte is not mainly controlled by the OH adsorption. Therefore, a bifunctional catalyst promoting OH adsorption may not useful for HOR in alkaline electrolyte. Tuning the hydrogen binding energy was found to be an efficient way to enhance the HOR activity, and making Pt base alloy is a reasonable way to tune the hydrogen binding energies.
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Cites
Origin of the Overpotential for Oxygen Reduction at a Fuel-Cell Cathode
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Cited by
Zheng, Y., Jiao, Y., Vasileff, A., & Qiao, S. (2018) · Angewandte Chemie International Edition · doi:10.1002/anie.201710556 · Cited by 1,489
Anion exchange membrane fuel cells: Current status and remaining challenges
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Hydrogen Evolution and Oxidation: Mechanistic Studies and Material Advances
Tian, X., Zhao, P., & Sheng, W. (2019) · Advanced Materials · doi:10.1002/adma.201808066 · Cited by 751
Diao, J., Qiu, Y., Liu, S., Wang, W., Chen, K., Li, H., Yuan, W., Qu, Y., & Guo, X. (2020) · Advanced Materials · doi:10.1002/adma.201905679 · Cited by 555
Strategies for design of electrocatalysts for hydrogen evolution under alkaline conditions
Wang, X., Zheng, Y., Sheng, W., Xu, Z. J., Jaroniec, M., & Qiao, S.-Z. (2020) · Materials Today · doi:10.1016/j.mattod.2019.12.003 · Cited by 533
Metadata
- Authors
- Lu, S., & Zhuang, Z.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2017-03-29
- Volume
- 139
- Issue
- 14
- Pages
- 5156-5163
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2603625925
- Cited by
- 340
- References
- 14
- FWCI
- 7.04
- Type
- journal article
- Language
- en
- Open access
- closed
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- Lu, S., & Zhuang, Z. (2017). Investigating the Influences of the Adsorbed Species on Catalytic Activity for Hydrogen Oxidation Reaction in Alkaline Electrolyte. Journal of the American Chemical Society. https://doi.org/10.1021/jacs.7b00765
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