The DOI matches its Crossref record; 2 of the 2 references it cites were found in a registry or an index.
Ammonia Electrosynthesis with High Selectivity under Ambient Conditions via a Li+ Incorporation Strategy
Abstract
We report the discovery of a dramatically enhanced N 2 electroreduction reaction (NRR) selectivity under ambient conditions via the Li + incorporation into poly( N -ethyl-benzene-1,2,4,5-tetracarboxylic diimide) (PEBCD) as a catalyst. The detailed electrochemical evaluation and density functional theory calculations showed that Li + association with the O atoms in the PEBCD matrix can retard the HER process and can facilitate the adsorption of N 2 to afford a high potential scope for the NRR process to proceed in the “[O—Li + ]·N 2 —H x ” alternating hydrogenation mode. This atomic-scale incorporation strategy provides new insight into the rational design of NRR catalysts with higher selectivity.
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Cites
Combining theory and experiment in electrocatalysis: Insights into materials design
Seh, Z. W., Kibsgaard, J., Dickens, C. F., Chorkendorff, I., Nørskov, J. K., & Jaramillo, T. F. (2017) · Science · doi:10.1126/science.aad4998 · Cited by 12,114
Review of electrochemical ammonia production technologies and materials
Giddey, S., Badwal, S. P. S., & Kulkarni, A. (2013) · International Journal of Hydrogen Energy · doi:10.1016/j.ijhydene.2013.09.054 · Cited by 886
Cited by
Wang, Y., Zhou, W., Jia, R., Yu, Y., & Zhang, B. (2020) · Angewandte Chemie International Edition · doi:10.1002/anie.201915992 · Cited by 1,641
A Review of Electrocatalytic Reduction of Dinitrogen to Ammonia under Ambient Conditions
Cui, X., Tang, C., & Zhang, Q. (2018) · Advanced Energy Materials · doi:10.1002/aenm.201800369 · Cited by 1,314
A review of ammonia as a compression ignition engine fuel
Dimitriou, P., & Javaid, R. (2020) · International Journal of Hydrogen Energy · doi:10.1016/j.ijhydene.2019.12.209 · Cited by 991
Geng, Z., Liu, Y., Kong, X., Li, P., Li, K., Liu, Z., Du, J., Shu, M., Si, R., & Zeng, J. (2018) · Advanced Materials · doi:10.1002/adma.201803498 · Cited by 913
Efficient Electrocatalytic N2 Fixation with MXene under Ambient Conditions
Luo, Y., Chen, G.-F., Ding, L., Chen, X., Ding, L.-X., & Wang, H. (2019) · Joule · doi:10.1016/j.joule.2018.09.011 · Cited by 699
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Metadata
- Authors
- Chen, G.-F., Cao, X., Wu, S., Zeng, X., Ding, L.-X., Zhu, M., & Wang, H.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2017-07-13
- Volume
- 139
- Issue
- 29
- Pages
- 9771-9774
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2735489250
- Cited by
- 626
- References
- 2
- FWCI
- 23.92
- Type
- journal article
- Language
- en
- Open access
- closed
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- Chen, G.-F., Cao, X., Wu, S., Zeng, X., Ding, L.-X., Zhu, M., & Wang, H. (2017). Ammonia Electrosynthesis with High Selectivity under Ambient Conditions via a Li+ Incorporation Strategy. Journal of the American Chemical Society. https://doi.org/10.1021/jacs.7b04393
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