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Construction of ZnIn2S4–In2O3 Hierarchical Tubular Heterostructures for Efficient CO2 Photoreduction
Abstract
We demonstrate the rational design and construction of sandwich-like ZnIn 2 S 4 –In 2 O 3 hierarchical tubular heterostructures by growing ZnIn 2 S 4 nanosheets on both inner and outer surfaces of In 2 O 3 microtubes as photocatalysts for efficient CO 2 photoreduction. The unique design integrates In 2 O 3 and ZnIn 2 S 4 into hierarchical one-dimensional (1D) open architectures with double-heterojunction shells and ultrathin two-dimensional (2D) nanosheet subunits. This design accelerates the separation and transfer of photogenerated charges, offers large surface area for CO 2 adsorption, and exposes abundant active sites for surface catalysis. Benefiting from the structural and compositional merits, the optimized ZnIn 2 S 4 –In 2 O 3 photocatalyst exhibits outstanding performance for reductive CO 2 deoxygenation with considerable CO generation rate (3075 μmol h –1 g –1 ) and high stability.
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Cited by
Vu, N., Kaliaguine, S., & Do, T. (2019) · Advanced Functional Materials · doi:10.1002/adfm.201901825 · Cited by 445
Li, B., Lai, C., Zeng, G., Huang, D., Qin, L., Zhang, M., Cheng, M., Liu, X., Yi, H., Zhou, C., et al. (2019) · Small · doi:10.1002/smll.201804565 · Cited by 367
Enabling Specific Photocatalytic Methane Oxidation by Controlling Free Radical Type
Jiang, Y., Li, S., Wang, S., Zhang, Y., Long, C., Xie, J., Fan, X., Zhao, W., Xu, P., Fan, Y., et al. (2023) · Journal of the American Chemical Society · doi:10.1021/jacs.2c13313 · Cited by 341
Self-citationChai, L., Hu, Z., Wang, X., Xu, Y., Zhang, L., Li, T., Hu, Y., Qian, J., & Huang, S. (2020) · Advanced Science · doi:10.1002/advs.201903195 · Cited by 296
Wang, Y., Wang, S., & Lou, X. W. (. (2019) · Angewandte Chemie International Edition · doi:10.1002/anie.201909707 · Cited by 237
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Metadata
- Authors
- Wang, S., Guan, B. Y., & Lou, X. W. D.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2018-03-29
- Volume
- 140
- Issue
- 15
- Pages
- 5037-5040
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2794692883
- Cited by
- 1,218
- References
- 0
- FWCI
- 28.22
- Type
- journal article
- Language
- en
- Open access
- closed
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- Wang, S., Guan, B. Y., & Lou, X. W. D. (2018). Construction of ZnIn2S4–In2O3 Hierarchical Tubular Heterostructures for Efficient CO2 Photoreduction. Journal of the American Chemical Society. https://doi.org/10.1021/jacs.8b02200
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