The DOI matches its Crossref record; 4 of the 4 references it cites were found in a registry or an index.
Photoreforming of Nonrecyclable Plastic Waste over a Carbon Nitride/Nickel Phosphide Catalyst
Open accessAbstract
Abstract With over 8 billion tons of plastic produced since 1950, polymers represent one of the most widely used─and most widely discarded─materials. Ambient-temperature photoreforming offers a simple and low-energy means for transforming plastic waste into fuel and bulk chemicals but has previously only been reported using precious-metal- or Cd-based photocatalysts. Here, an inexpensive and nontoxic carbon nitride/nickel phosphide (CNx|Ni2P) photocatalyst is utilized to successfully reform poly(ethylene terephthalate) (PET) and poly(lactic acid) (PLA) to clean H2 fuel and a variety of organic chemicals under alkaline aqueous conditions. Ni2P synthesized on cyanamide-functionalized carbon nitride is shown to promote efficient charge separation and catalysis, with a photostability of at least 5 days. The real-world applicability of photoreforming is further verified by generating H2 and organics from a selection of nonrecyclable waste─including microplastics (polyester microfibers) and food-contaminated plastic─and upscaling the system from 2 to 120 mL while maintaining its efficiency for plastic conversion.
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Production, use, and fate of all plastics ever made
Geyer, R., Jambeck, J. R., & Law, K. L. (2017) · Science Advances · doi:10.1126/sciadv.1700782 · Cited by 18,606
Metal-free efficient photocatalyst for stable visible water splitting via a two-electron pathway
Liu, J., Liu, Y., Liu, N., Han, Y., Zhang, X., Huang, H., Lifshitz, Y., Lee, S.-T., Zhong, J., & Kang, Z. (2015) · Science · doi:10.1126/science.aaa3145 · Cited by 4,468
Plastic debris in the open ocean
Cózar, A., Echevarría, F., González-Gordillo, J. I., Irigoien, X., Úbeda, B., Hernández-León, S., Palma, Á. T., Navarro, S., García-de-Lomas, J., Ruiz, A., et al. (2014) · Proceedings of the National Academy of Sciences · doi:10.1073/pnas.1314705111 · Cited by 3,133
Recent advances in the gasification of waste plastics. A critical overview
Lopez, G., Artetxe, M., Amutio, M., Alvarez, J., Bilbao, J., & Olazar, M. (2018) · Renewable and Sustainable Energy Reviews · doi:10.1016/j.rser.2017.09.032 · Cited by 852
Cited by
Beyond Mechanical Recycling: Giving New Life to Plastic Waste
Vollmer, I., Jenks, M. J. F., Roelands, M. C. P., White, R. J., van Harmelen, T., de Wild, P., van der Laan, G. P., Meirer, F., Keurentjes, J. T. F., & Weckhuysen, B. M. (2020) · Angewandte Chemie International Edition · doi:10.1002/anie.201915651 · Cited by 1,905
Bifunctional Electrocatalysts for Overall and Hybrid Water Splitting
Quan, L., Jiang, H., Mei, G., Sun, Y., & You, B. (2024) · Chemical Reviews · doi:10.1021/acs.chemrev.3c00332 · Cited by 874
Upcycling and catalytic degradation of plastic wastes
Hou, Q., Zhen, M., Qian, H., Nie, Y., Bai, X., Xia, T., Laiq Ur Rehman, M., Li, Q., & Ju, M. (2021) · Cell Reports Physical Science · doi:10.1016/j.xcrp.2021.100514 · Cited by 335
Gunawan, D., Zhang, J., Li, Q., Toe, C. Y., Scott, J., Antonietti, M., Guo, J., & Amal, R. (2024) · Advanced Materials · doi:10.1002/adma.202404618 · Cited by 325
Recent Progress in the Chemical Upcycling of Plastic Wastes
Chen, X., Wang, Y., & Zhang, L. (2021) · ChemSusChem · doi:10.1002/cssc.202100868 · Cited by 298
Metadata
- Authors
- Uekert, T., Kasap, H., & Reisner, E.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2019-08-29
- Volume
- 141
- Issue
- 38
- Pages
- 15201-15210
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2970296536
- Cited by
- 697
- References
- 4
- FWCI
- 8.81
- Type
- journal article
- Language
- en
- Open access
- hybrid
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- Uekert, T., Kasap, H., & Reisner, E. (2019). Photoreforming of Nonrecyclable Plastic Waste over a Carbon Nitride/Nickel Phosphide Catalyst. Journal of the American Chemical Society. https://doi.org/10.1021/jacs.9b06872
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