The DOI matches its Crossref record; 2 of the 2 references it cites were found in a registry or an index.
Scalable and Template-Free Aqueous Synthesis of Zirconium-Based Metal–Organic Framework Coating on Textile Fiber
Abstract
Organophosphonate-based nerve agents, such as VX, Sarin (GB), and Soman (GD), are among the most toxic chemicals to humankind. Recently, we have shown that Zr-based metal-organic frameworks (Zr-MOFs) can effectively catalyze the hydrolysis of these toxic chemicals for diminishing their toxicity. On the other hand, utilizing these materials in powder form is not practical, and developing scalable and economical processes for integrating these materials onto fibers is crucial for protective gear. Herein, we report a scalable, template-free, and aqueous solution-based synthesis strategy for the production of Zr-MOF-coated textiles. Among all MOF/fiber composites reported to date, the MOF-808/polyester fibers exhibit the highest rates of nerve agent hydrolysis. Moreover, such highly porous fiber composites display significantly higher protection time compared to that of its parent fabric for a mustard gas simulant, 2-chloroethyl ethyl sulfide (CEES). A decreased diffusion rate of toxic chemicals through the MOF layer can provide time needed for the destruction of the harmful species.
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Cites
Metal-organic framework materials as catalysts
Lee, J., Farha, O. K., Roberts, J., Scheidt, K. A., Nguyen, S. T., & Hupp, J. T. (2009) · Chemical Society Reviews · doi:10.1039/b807080f · Cited by 7,969
Self-citationAcetylcholinesterase Inhibitors: Pharmacology and Toxicology
Colovic, M. B., Krstic, D. Z., Lazarevic-Pasti, T. D., Bondzic, A. M., & Vasic, V. M. (2013) · Current Neuropharmacology · doi:10.2174/1570159x11311030006 · Cited by 2,611
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Metal–Organic Framework-Based Catalysts with Single Metal Sites
Wei, Y.-S., Zhang, M., Zou, R., & Xu, Q. (2020) · Chemical Reviews · doi:10.1021/acs.chemrev.9b00757 · Cited by 1,233
Metal–Organic Frameworks against Toxic Chemicals
Islamoglu, T., Chen, Z., Wasson, M. C., Buru, C. T., Kirlikovali, K. O., Afrin, U., Mian, M. R., & Farha, O. K. (2020) · Chemical Reviews · doi:10.1021/acs.chemrev.9b00828 · Cited by 707
Self-citationElectronic Textiles for Wearable Point-of-Care Systems
Chen, G., Xiao, X., Zhao, X., Tat, T., Bick, M., & Chen, J. (2022) · Chemical Reviews · doi:10.1021/acs.chemrev.1c00502 · Cited by 688
Bioinspired Framework Catalysts: From Enzyme Immobilization to Biomimetic Catalysis
Wang, K.-Y., Zhang, J., Hsu, Y.-C., Lin, H., Han, Z., Pang, J., Yang, Z., Liang, R.-R., Shi, W., & Zhou, H.-C. (2023) · Chemical Reviews · doi:10.1021/acs.chemrev.2c00879 · Cited by 490
Kirlikovali, K. O., Chen, Z., Islamoglu, T., Hupp, J. T., & Farha, O. K. (2020) · ACS Applied Materials & Interfaces · doi:10.1021/acsami.9b20154 · Cited by 286
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Metadata
- Authors
- Ma, K., Islamoglu, T., Chen, Z., Li, P., Wasson, M. C., Chen, Y., Wang, Y., Peterson, G. W., Xin, J. H., & Farha, O. K.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2019-09-18
- Volume
- 141
- Issue
- 39
- Pages
- 15626-15633
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2974102229
- Cited by
- 209
- References
- 2
- FWCI
- 9.28
- Type
- journal article
- Language
- en
- Open access
- closed
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