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Oxygen Reduction on Silver Low-Index Single-Crystal Surfaces in Alkaline Solution: Rotating Ring DiskAg(hkl) Studies
Abstract
The rotating ring disk method is applied to investigate the oxygen reduction reaction on Ag single-crystal surfaces in alkaline solution over the temperature range 293-333 K. At all temperatures, the oxygen reduction reaction proceeds through the 4e- reaction pathway with a very small (approximately 0.5-2%) peroxide formation. At the same temperature and overpotentials, the kinetics of the ORR always increases in the order (100) < or = (111) < (110), indicating that the reaction is structure-sensitive. We present an interpretation of the structure sensitivity based on the supposition that it arises from (i) a potential-dependent adsorption of spectator hydroxyl ions and (ii) variations in activation energies, which are determined by the O2 adsorption on Ag single-crystal surfaces covered by adsorbed oxygenated species.
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Markovic, N. M., Gasteiger, H. A., & Ross, P. N. (1995) · The Journal of Physical Chemistry · doi:10.1021/j100011a001 · Cited by 736
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Cited by
Shinagawa, T., Garcia-Esparza, A. T., & Takanabe, K. (2015) · Scientific Reports · doi:10.1038/srep13801 · Cited by 3,287
Oxygen Reduction in Alkaline Media: From Mechanisms to Recent Advances of Catalysts
Ge, X., Sumboja, A., Wuu, D., An, T., Li, B., Goh, F. W. T., Hor, T. S. A., Zong, Y., & Liu, Z. (2015) · ACS Catalysis · doi:10.1021/acscatal.5b00524 · Cited by 1,341
Active and stable carbon nanotube/nanoparticle composite electrocatalyst for oxygen reduction
Chung, H. T., Won, J. H., & Zelenay, P. (2013) · Nature Communications · doi:10.1038/ncomms2944 · Cited by 820
Nanoparticle Silver Catalysts That Show Enhanced Activity for Carbon Dioxide Electrolysis
Salehi-Khojin, A., Jhong, H.-R. M., Rosen, B. A., Zhu, W., Ma, S., Kenis, P. J. A., & Masel, R. I. (2013) · The Journal of Physical Chemistry C · doi:10.1021/jp310509z · Cited by 435
Slanac, D. A., Hardin, W. G., Johnston, K. P., & Stevenson, K. J. (2012) · Journal of the American Chemical Society · doi:10.1021/ja303580b · Cited by 295
Metadata
- Authors
- Blizanac, B. B., Ross, P. N., & Marković, N. M.
- Venue
- The Journal of Physical Chemistry B
- Publisher
- American Chemical Society (ACS)
- Published
- 2006-02-22
- Volume
- 110
- Issue
- 10
- Pages
- 4735-4741
- ISSN
- 1520-5207 (ISSN-L)
- 1520-6106
- OpenAlex
- W1965636614
- Cited by
- 317
- References
- 1
- FWCI
- 3.84
- Type
- journal article
- Language
- en
- Open access
- closed
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- Blizanac, B. B., Ross, P. N., & Marković, N. M. (2006). Oxygen Reduction on Silver Low-Index Single-Crystal Surfaces in Alkaline Solution: Rotating Ring DiskAg(hkl) Studies. The Journal of Physical Chemistry B. https://doi.org/10.1021/jp056050d
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