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Far-Infrared Dielectric Properties of Polar Liquids Probed by Femtosecond Terahertz Pulse Spectroscopy
Abstract
We report the frequency-dependent optical constants, n (ν) and α(ν), or, equivalently, the complex permittivity ε(ω) = ε‘(ω) − iε‘‘(ω), over the frequency range from 2 to 50 cm -1 for water, methanol, ethanol, 1-propanol, and liquid ammonia. These spectra have been measured with femtosecond terahertz pulse transmission spectroscopy. These liquids exhibit multiple-Debye behavior, making their frequency-dependent dielectric constants valuable benchmarks for molecular dynamics simulations and other theoretical treatments of liquids.
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Cites
Characterization of an optoelectronic terahertz beam system
van Exter, M., & Grischkowsky, D. R. (1990) · IEEE Transactions on Microwave Theory and Techniques · doi:10.1109/22.60016 · Cited by 486
Cited by
Terahertz spectroscopy and imaging - Modern techniques and applications
Jepsen, P. U., Cooke, D. G., & Koch, M. (2011) · Laser & Photonics Reviews · doi:10.1002/lpor.201000011 · Cited by 2,091
Terahertz Technology in Biology and Medicine
Siegel, P. H. (2004) · IEEE Transactions on Microwave Theory and Techniques · doi:10.1109/tmtt.2004.835916 · Cited by 1,378
Imaging with terahertz radiation
Chan, W. L., Deibel, J., & Mittleman, D. M. (2007) · Reports on Progress in Physics · doi:10.1088/0034-4885/70/8/r02 · Cited by 965
A simple polarizable model of water based on classical Drude oscillators
Lamoureux, G., MacKerell, A. D., & Roux, B. (2003) · The Journal of Chemical Physics · doi:10.1063/1.1598191 · Cited by 688
Tutorial: An introduction to terahertz time domain spectroscopy (THz-TDS)
Neu, J., & Schmuttenmaer, C. A. (2018) · Journal of Applied Physics · doi:10.1063/1.5047659 · Cited by 675
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Metadata
- Authors
- Kindt, J. T., & Schmuttenmaer, C. A.
- Venue
- The Journal of Physical Chemistry
- Publisher
- American Chemical Society (ACS)
- Published
- 1996-01-01
- Volume
- 100
- Issue
- 24
- Pages
- 10373-10379
- ISSN
- 0022-3654 (ISSN-L)
- 1541-5740
- OpenAlex
- W2005420127
- Cited by
- 687
- References
- 1
- FWCI
- 20.39
- Type
- journal article
- Language
- en
- Open access
- closed
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- Kindt, J. T., & Schmuttenmaer, C. A. (1996). Far-Infrared Dielectric Properties of Polar Liquids Probed by Femtosecond Terahertz Pulse Spectroscopy. The Journal of Physical Chemistry. https://doi.org/10.1021/jp960141g
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