The DOI matches its Crossref record; 1 of the 1 references it cites were found in a registry or an index.
Dynamics of Lithium Dendrite Growth and Inhibition: Pulse Charging Experiments and Monte Carlo Calculations
Abstract
Short-circuiting via dendrites compromises the reliability of Li-metal batteries. Dendrites ensue from instabilities inherent to electrodeposition that should be amenable to dynamic control. Here, we report that by charging a scaled coin-cell prototype with 1 ms pulses followed by 3 ms rest periods the average dendrite length is shortened ∼2.5 times relative to those grown under continuous charging. Monte Carlo simulations dealing with Li(+) diffusion and electromigration reveal that experiments involving 20 ms pulses were ineffective because Li(+) migration in the strong electric fields converging to dendrite tips generates extended depleted layers that cannot be replenished by diffusion during rest periods. Because the application of pulses much shorter than the characteristic time τc ∼ O(∼1 ms) for polarizing electric double layers in our system would approach DC charging, we suggest that dendrite propagation can be inhibited (albeit not suppressed) by pulse charging within appropriate frequency ranges.
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Cites
Orsini, F., Du Pasquier, A., Beaudoin, B., Tarascon, J. M., Trentin, M., Langenhuizen, N., De Beer, E., & Notten, P. (1998) · Journal of Power Sources · doi:10.1016/s0378-7753(98)00128-1 · Cited by 310
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Tomaszewska, A., Chu, Z., Feng, X., O'Kane, S., Liu, X., Chen, J., Ji, C., Endler, E., Li, R., Liu, L., et al. (2019) · eTransportation · doi:10.1016/j.etran.2019.100011 · Cited by 1,592
Mechanism of Lithium Metal Penetration through Inorganic Solid Electrolytes
Porz, L., Swamy, T., Sheldon, B. W., Rettenwander, D., Frömling, T., Thaman, H. L., Berendts, S., Uecker, R., Carter, W. C., & Chiang, Y. (2017) · Advanced Energy Materials · doi:10.1002/aenm.201701003 · Cited by 1,117
Li plating as unwanted side reaction in commercial Li-ion cells – A review
Waldmann, T., Hogg, B.-I., & Wohlfahrt-Mehrens, M. (2018) · Journal of Power Sources · doi:10.1016/j.jpowsour.2018.02.063 · Cited by 895
Self-heating–induced healing of lithium dendrites
Li, L., Basu, S., Wang, Y., Chen, Z., Hundekar, P., Wang, B., Shi, J., Shi, Y., Narayanan, S., & Koratkar, N. (2018) · Science · doi:10.1126/science.aap8787 · Cited by 528
Lithium Plating Mechanism, Detection, and Mitigation in Lithium-Ion Batteries
Lin, X., Khosravinia, K., Hu, X., Li, J., & Lu, W. (2021) · Progress in Energy and Combustion Science · doi:10.1016/j.pecs.2021.100953 · Cited by 490
Metadata
- Authors
- Aryanfar, A., Brooks, D., Merinov, B. V., Goddard, W. A., Colussi, A. J., & Hoffmann, M. R.
- Venue
- The Journal of Physical Chemistry Letters
- Publisher
- American Chemical Society (ACS)
- Published
- 2014-05-02
- Volume
- 5
- Issue
- 10
- Pages
- 1721-1726
- ISSN
- 1948-7185 (ISSN-L)
- OpenAlex
- W2136541759
- Cited by
- 226
- References
- 1
- FWCI
- 5.84
- Type
- journal article
- Language
- en
- Open access
- closed
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
