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Plasmonic Photoanodes for Solar Water Splitting with Visible Light
Abstract
We report a plasmonic water splitting cell in which 95% of the effective charge carriers derive from surface plasmon decay to hot electrons, as evidenced by fuel production efficiencies up to 20-fold higher at visible, as compared to UV, wavelengths. The cell functions by illuminating a dense array of aligned gold nanorods capped with TiO(2), forming a Schottky metal/semiconductor interface which collects and conducts the hot electrons to an unilluminated platinum counter-electrode where hydrogen gas evolves. The resultant positive charges in the Au nanorods function as holes and are extracted by an oxidation catalyst which electrocatalytically oxidizes water to oxygen gas.
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Titanium dioxide for solar-hydrogen I. Functional properties☆
NOWOTNY, J., BAK, T., NOWOTNY, M., & SHEPPARD, L. (2007) · International Journal of Hydrogen Energy · doi:10.1016/j.ijhydene.2006.09.004 · Cited by 214
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Metadata
- Authors
- Lee, J., Mubeen, S., Ji, X., Stucky, G. D., & Moskovits, M.
- Venue
- Nano Letters
- Publisher
- American Chemical Society (ACS)
- Published
- 2012-08-27
- Volume
- 12
- Issue
- 9
- Pages
- 5014-5019
- ISSN
- 1530-6984 (ISSN-L)
- 1530-6992
- OpenAlex
- W1980749521
- Cited by
- 539
- References
- 2
- FWCI
- 16.40
- Type
- journal article
- Language
- en
- Open access
- closed
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
