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Thermal Conduction in Aligned Carbon Nanotube–Polymer Nanocomposites with High Packing Density

Marconnet, Amy M., Yamamoto, Namiko, Panzer, Matthew A., Wardle, Brian L., Goodson, Kenneth E.·2011·ACS Nano

Abstract

Nanostructured composites containing aligned carbon nanotubes (CNTs) are very promising as interface materials for electronic systems and thermoelectric power generators. We report the first data for the thermal conductivity of densified, aligned multiwall CNT nanocomposite films for a range of CNT volume fractions. A 1 vol % CNT composite more than doubles the thermal conductivity of the base polymer. Denser arrays (17 vol % CNTs) enhance the thermal conductivity by as much as a factor of 18 and there is a nonlinear trend with CNT volume fraction. This article discusses the impact of CNT density on thermal conduction considering boundary resistances, increased defect concentrations, and the possibility of suppressed phonon modes in the CNTs.

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Crossref · 10.1021/nn200847u

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Metadata

Authors
Marconnet, A. M., Yamamoto, N., Panzer, M. A., Wardle, B. L., & Goodson, K. E.
Affiliations
  • Department of Mechanical Engineering, Building 530, Room 224, 440 Escondido Mall, Stanford University, Stanford, California 94305, United States
  • Department of Aeronautics and Astronautics, Room 41-317, 77 Massachusetts Avenue, Massachusetts Institute of Technology, Cambridge, Massachusetts 02139, United States
Venue
ACS Nano
Published
2011-06-03
Volume
5
Issue
6
Pages
4818-4825
ISSN
  • 1936-0851
  • 1936-086X
Cited by
474
References
1
Language
en

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