The DOI matches its Crossref record; 6 of the 6 references it cites were found in a registry or an index.
Fibrous Hybrid of Graphene and Sulfur Nanocrystals for High-Performance Lithium–Sulfur Batteries
Abstract
Graphene-sulfur (G-S) hybrid materials with sulfur nanocrystals anchored on interconnected fibrous graphene are obtained by a facile one-pot strategy using a sulfur/carbon disulfide/alcohol mixed solution. The reduction of graphene oxide and the formation/binding of sulfur nanocrystals were integrated. The G-S hybrids exhibit a highly porous network structure constructed by fibrous graphene, many electrically conducting pathways, and easily tunable sulfur content, which can be cut and pressed into pellets to be directly used as lithium-sulfur battery cathodes without using a metal current-collector, binder, and conductive additive. The porous network and sulfur nanocrystals enable rapid ion transport and short Li(+) diffusion distance, the interconnected fibrous graphene provides highly conductive electron transport pathways, and the oxygen-containing (mainly hydroxyl/epoxide) groups show strong binding with polysulfides, preventing their dissolution into the electrolyte based on first-principles calculations. As a result, the G-S hybrids show a high capacity, an excellent high-rate performance, and a long life over 100 cycles. These results demonstrate the great potential of this unique hybrid structure as cathodes for high-performance lithium-sulfur batteries.
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Cites
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Cited by
Wang, Z., Dong, Y., Li, H., Zhao, Z., Bin Wu, H., Hao, C., Liu, S., Qiu, J., & Lou, X. W. (2014) · Nature Communications · doi:10.1038/ncomms6002 · Cited by 1,059
Graphene and Graphene‐Based Materials for Energy Storage Applications
Zhu, J., Yang, D., Yin, Z., Yan, Q., & Zhang, H. (2014) · Small · doi:10.1002/smll.201303202 · Cited by 825
Pei, F., An, T., Zang, J., Zhao, X., Fang, X., Zheng, M., Dong, Q., & Zheng, N. (2016) · Advanced Energy Materials · doi:10.1002/aenm.201502539 · Cited by 555
Xu, J., Ma, J., Fan, Q., Guo, S., & Dou, S. (2017) · Advanced Materials · doi:10.1002/adma.201606454 · Cited by 319
Lin, Y., Lai, S., & Wu, J. M. (2020) · Advanced Materials · doi:10.1002/adma.202002875 · Cited by 131
Metadata
- Authors
- Zhou, G., Yin, L.-C., Wang, D.-W., Li, L., Pei, S., Gentle, I. R., Li, F., & Cheng, H.-M.
- Venue
- ACS Nano
- Publisher
- American Chemical Society (ACS)
- Published
- 2013-05-16
- Volume
- 7
- Issue
- 6
- Pages
- 5367-5375
- ISSN
- 1936-0851 (ISSN-L)
- 1936-086X
- OpenAlex
- W2087001279
- Cited by
- 761
- References
- 6
- FWCI
- 48.93
- Type
- journal article
- Language
- en
- Open access
- closed
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- Zhou, G., Yin, L.-C., Wang, D.-W., Li, L., Pei, S., Gentle, I. R., Li, F., & Cheng, H.-M. (2013). Fibrous Hybrid of Graphene and Sulfur Nanocrystals for High-Performance Lithium–Sulfur Batteries. ACS Nano. https://doi.org/10.1021/nn401228t
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