The DOI matches its Crossref record; 41 of the 41 references it cites were found in a registry or an index.
On the Dynamics of Charging in Nanoporous Carbon-Based Supercapacitors
Open accessAbstract
Supercapacitors are electricity storage systems with high power performances. Their short charge/discharge times are due to fast adsorption/desorption rates for the ions of the electrolyte on the electrode surface. Nanoporous carbon electrodes, which give larger capacitances than simpler geometries, might be expected to show poorer power performances because of the longer times taken by the ions to access the electrode interior. Experiments do not show such trends, however, and this remains to be explained at the molecular scale. Here we show that carbide-derived carbons exhibit heterogeneous and fast charging dynamics. We perform molecular dynamics simulations, with realistically modeled nanoporous electrodes and an ionic liquid electrolyte, in which the system, originally at equilibrium in the uncharged state, is suddenly perturbed by the application of an electric potential difference between the electrodes. The electrodes respond by charging progressively from the interface to the bulk as ions are exchanged between the nanopores and the electrolyte region. The simulation results are then injected into an equivalent circuit model, which allows us to calculate charging times for macroscopic-scale devices.
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Cites
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Self-citationElectrochemical Supercapacitors : Scientific Fundamentals and Technological Applications
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Self-citationAnomalous Increase in Carbon Capacitance at Pore Sizes Less Than 1 Nanometer
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Self-citationElectrochemical Supercapacitors
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Self-citationElectrochemical Characteristics and Impedance Spectroscopy Studies of Carbon-Carbon Supercapacitors
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Self-citationLiquid-Mediated Dense Integration of Graphene Materials for Compact Capacitive Energy Storage
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Cited by
Efficient storage mechanisms for building better supercapacitors
Salanne, M., Rotenberg, B., Naoi, K., Kaneko, K., Taberna, P.-L., Grey, C. P., Dunn, B., & Simon, P. (2016) · Nature Energy · doi:10.1038/nenergy.2016.70 · Cited by 2,181
Self-citationZhang, S., Zhang, J., Zhang, Y., & Deng, Y. (2017) · Chemical Reviews · doi:10.1021/acs.chemrev.6b00509 · Cited by 659
Revitalizing carbon supercapacitor electrodes with hierarchical porous structures
Liu, T., Zhang, F., Song, Y., & Li, Y. (2017) · Journal of Materials Chemistry A · doi:10.1039/c7ta05646j · Cited by 621
Microscopic Simulations of Electrochemical Double-Layer Capacitors
Jeanmairet, G., Rotenberg, B., & Salanne, M. (2022) · Chemical Reviews · doi:10.1021/acs.chemrev.1c00925 · Cited by 303
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Metadata
- Authors
- Péan, C., Merlet, C., Rotenberg, B., Madden, P. A., Taberna, P.-L., Daffos, B., Salanne, M., & Simon, P.
- Venue
- ACS Nano
- Publisher
- American Chemical Society (ACS)
- Published
- 2014-01-15
- Volume
- 8
- Issue
- 2
- Pages
- 1576-1583
- ISSN
- 1936-0851 (ISSN-L)
- 1936-086X
- OpenAlex
- W1998873401
- Cited by
- 253
- References
- 41
- FWCI
- 7.74
- Type
- journal article
- Language
- en
- Open access
- green
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Bibliographic data: Semantic Scholar, OpenAlex, Crossref.
Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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