Supramolecular Hydrogel of Chitosan in the Presence of Graphene Oxide Nanosheets as 2D Cross-Linkers
Abstract
Biomass-based materials are attractive due to their renewability, biodegradability, and biocompatibility. Chitosan is a typical biomacromolecule that can be used as feedstock for novel materials. Here, the self-assembly of chitosan chains with graphene oxide (GO) nanosheets has been studied, where GO works as the two-dimensional cross-linker dues to its multifunctional groups on both sides. Supramolecular hydrogels of chitosan and GO have been prepared by controlling the concentration of GO, ratio of chitosan to GO, and temperature. It was found that at high GO concentration, hydrogel can be obtained at room temperature, and the as-prepared hydrogel showed a self-healing performance. However, at low GO concentration, the supramolecular hydrogel formed only at high temperature (95 °C). The driving force for the hydrogel is believed to be the noncovalent interactions. The reversible hydrogels have potential applications in fields of biomaterials, wastewater treatment, and smart materials.
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The beneficial influence of GO is related to the mechanical stability of the CS-GO supports, maintaining surface area and porosity, thereby giving a better metal-support interaction with the Pd nanoparticles.
“According to the literature [27], the beneficial influence of GO should be related to the mechanical stability of the CS-GO supports, maintaining surface area and porosity, thereby having a better metal-support interaction with the Pd NPs.”
From Palladium Supported on Porous Chitosan–Graphene Oxide Aerogels as Highly Efficient Catalysts for Hydrogen Generation from Formate (2019) · cites this paper as [27]
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- Authors
- Han, D., & Yan, L.
- Affiliations
- University of Science and Technology of China (CN)
- Corresponding author
- Yan, Lifeng
- Venue
- ACS Sustainable Chemistry & Engineering
- Publisher
- American Chemical Society (ACS)
- Published
- 2013-10-09
- Volume
- 2
- Issue
- 2
- Pages
- 296-300
- ISSN
- 2168-0485 (ISSN-L)
- OpenAlex
- W2315517520
- Cited by
- 130
- References
- 29
- Citations by year
- 2026: 2 · 2025: 7 · 2024: 9 · 2023: 5 · 2022: 11 · 2021: 13 · 2020: 12 · 2019: 7 · 2018: 19 · 2017: 13 · 2016: 16 · 2015: 11 · 2014: 5
- FWCI
- 4.07
- Type
- journal article
- Language
- en
- Open access
- closed
- Locations
- ACS Sustainable Chemistry & Engineering (publishedVersion)
- Topics
- Physical Sciences › Materials Science › Biomaterials › Supramolecular Self-Assembly in Materials
- Life Sciences › Biochemistry, Genetics and Molecular Biology › Molecular Medicine › Hydrogels: synthesis, properties, applications
- Physical Sciences › Materials Science › Biomaterials › Nanocomposite Films for Food Packaging
- Keywords
- chitosan, graphene oxide nanosheets, supramolecular hydrogels, self-assembly, self-healing hydrogels, non-covalent interactions, biomass-derived materials
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