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Colloidal lead halide perovskite nanocrystals: synthesis, optical properties and applications
Open accessAbstract
Lead halide perovskite nanocrystals (NCs) are receiving a lot of attention nowadays, due to their exceptionally high photoluminescence quantum yields reaching almost 100% and tunability of their optical band gap over the entire visible spectral range by modifying composition or dimensionality/size. We review recent developments in the direct synthesis and ion exchange-based reactions, leading to hybrid organic–inorganic (CH3NH3PbX3) and all-inorganic (CsPbX3) lead halide (X=Cl, Br, I) perovskite NCs, and consider their optical properties related to quantum confinement effects, single emission spectroscopy and lasing. We summarize recent developments on perovskite NCs employed as an active material in several applications such as light-emitting devices, solar cells and photodetectors, and provide a critical outlook into the existing and future challenges. Although research into perovskite nanocrystals is still in its infancy, they are expected to be major players in future nanoscience. Lead halide perovskite nanocrystals are attracting much interest because their quantum yields for photoluminescence are approaching 100% and their optical band gap can be tuned over the entire visible wavelength region – properties that make them promising for use in lasers, light-emitting diodes (LEDs) and solar cells. Andrey Rogach of City University of Hong Kong and co-workers review the latest developments in the synthesis (of both hybrid organic-inorganic and all-inorganic nanocrystals), optical properties (quantum confinement effects, single particle emission and lasing studies) and applications (LEDs, solar cells and photodiodes) of these materials. They outline some of the many remaining challenges, but state their confidence that these should soon be overcome. This review summarizes recent developments in the direct synthesis and ion exchange-based reactions leading to hybrid organic–inorganic and all-inorganic lead halide perovskite nanocrystals. Optical properties related to quantum confinement effects, single emission spectroscopy and lasing are considered. Perovskite nanocrystals have been employed as an active material in several applications such as light-emitting devices, solar cells and photodetectors.
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Kim, H.-S., Lee, C.-R., Im, J.-H., Lee, K.-B., Moehl, T., Marchioro, A., Moon, S.-J., Humphry-Baker, R., Yum, J.-H., Moser, J. E., et al. (2012) · Scientific Reports · doi:10.1038/srep00591 · Cited by 8,092
Lead halide perovskite nanowire lasers with low lasing thresholds and high quality factors
Zhu, H., Fu, Y., Meng, F., Wu, X., Gong, Z., Ding, Q., Gustafsson, M. V., Trinh, M. T., Jin, S., & Zhu, X.-Y. (2015) · Nature Materials · doi:10.1038/nmat4271 · Cited by 2,836
Akkerman, Q. A., D’Innocenzo, V., Accornero, S., Scarpellini, A., Petrozza, A., Prato, M., & Manna, L. (2015) · Journal of the American Chemical Society · doi:10.1021/jacs.5b05602 · Cited by 2,197
Deschler, F., Price, M., Pathak, S., Klintberg, L. E., Jarausch, D.-D., Higler, R., Hüttner, S., Leijtens, T., Stranks, S. D., Snaith, H. J., et al. (2014) · The Journal of Physical Chemistry Letters · doi:10.1021/jz5005285 · Cited by 1,753
Perovskite Microdisk Microlasers Self‐Assembled from Solution
Liao, Q., Hu, K., Zhang, H., Wang, X., Yao, J., & Fu, H. (2015) · Advanced Materials · doi:10.1002/adma.201500449 · Cited by 406
Cited by
Genesis, challenges and opportunities for colloidal lead halide perovskite nanocrystals
Akkerman, Q. A., Rainò, G., Kovalenko, M. V., & Manna, L. (2018) · Nature Materials · doi:10.1038/s41563-018-0018-4 · Cited by 2,287
Lead Halide Perovskite Nanocrystals in the Research Spotlight: Stability and Defect Tolerance
Huang, H., Bodnarchuk, M. I., Kershaw, S. V., Kovalenko, M. V., & Rogach, A. L. (2017) · ACS Energy Letters · doi:10.1021/acsenergylett.7b00547 · Cited by 1,236
Self-citationLow dimensional metal halide perovskites and hybrids
Zhou, C., Lin, H., He, Q., Xu, L., Worku, M., Chaaban, M., Lee, S., Shi, X., Du, M.-H., & Ma, B. (2019) · Materials Science and Engineering: R: Reports · doi:10.1016/j.mser.2018.12.001 · Cited by 489
Perovskite synthesis, properties and their related biochemical and industrial application
Assirey, E. A. R. (2019) · Saudi Pharmaceutical Journal · doi:10.1016/j.jsps.2019.05.003 · Cited by 445
Metal Halide Perovskite Light‐Emitting Devices: Promising Technology for Next‐Generation Displays
Lu, M., Zhang, Y., Wang, S., Guo, J., Yu, W. W., & Rogach, A. L. (2019) · Advanced Functional Materials · doi:10.1002/adfm.201902008 · Cited by 425
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Metadata
- Authors
- Huang, H., Polavarapu, L., Sichert, J. A., Susha, A. S., Urban, A. S., & Rogach, A. L.
- Venue
- NPG Asia Materials
- Published
- 2016-11
- Volume
- 8
- Issue
- 11
- Pages
- e328-e328
- ISSN
- 1884-4049 (ISSN-L)
- 1884-4057
- OpenAlex
- W2555716431
- Cited by
- 497
- References
- 5
- FWCI
- 27.59
- Type
- journal article
- Language
- en
- Open access
- gold
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