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Femtosecond electronic response of atoms to ultra-intense X-rays
Abstract
An era of exploring the interactions of high-intensity, hard X-rays with matter has begun with the start-up of a hard-X-ray free-electron laser, the Linac Coherent Light Source (LCLS). Understanding how electrons in matter respond to ultra-intense X-ray radiation is essential for all applications. Here we reveal the nature of the electronic response in a free atom to unprecedented high-intensity, short-wavelength, high-fluence radiation (respectively 10(18) W cm(-2), 1.5-0.6 nm, approximately 10(5) X-ray photons per A(2)). At this fluence, the neon target inevitably changes during the course of a single femtosecond-duration X-ray pulse-by sequentially ejecting electrons-to produce fully-stripped neon through absorption of six photons. Rapid photoejection of inner-shell electrons produces 'hollow' atoms and an intensity-induced X-ray transparency. Such transparency, due to the presence of inner-shell vacancies, can be induced in all atomic, molecular and condensed matter systems at high intensity. Quantitative comparison with theory allows us to extract LCLS fluence and pulse duration. Our successful modelling of X-ray/atom interactions using a straightforward rate equation approach augurs favourably for extension to complex systems.
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“the high number of photons comprising the ultrashort femtosecond pulses gives rise to the production of high charge states, which can only be explained by the absorption of many photons from the same pulse (e.g [1,74]).”
From Roadmap of ultrafast x-ray atomic and molecular physics (2018) · cites this paper as [1]
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Koulentianos, D., Fouda, A. E. A., Southworth, S. H., Bozek, J. D., Küpper, J., Santra, R., Kryzhevoi, N. V., Cederbaum, L. S., Bostedt, C., Messerschmidt, M. M., et al. (2020) · Journal of Physics B Atomic Molecular and Optical Physics · doi:10.1088/1361-6455/abc183 · Cited by 7
Self-citationResonance-enhanced x-ray multiple ionization of a polyatomic molecule
Li, X., Rudenko, A., Mazza, T., Rörig, A., Anders, N., Baumann, T., Eckart, S., Erk, B., Fanis, A. D., Fehre, K., et al. (2022) · Physical Review A · doi:10.1103/physreva.105.053102 · Cited by 7
On ultrafast x-ray scattering methods for magnetism
Plumley, R., Chitturi, S. R., Peng, C., Assefa, T. A., Burdet, N., Shen, L., Chen, Z., Reid, A. H., Dakovski, G. L., Seaberg, M., et al. (2024) · Advances in Physics X · doi:10.1080/23746149.2024.2423935 · Cited by 7
Kazansky, A. K., Sazhina, I. P., & Kabachnik, N. M. (2013) · Journal of Physics B Atomic Molecular and Optical Physics · doi:10.1088/0953-4075/46/2/025601 · Cited by 7
Isolated high-harmonic XUV photon absorption and NIR strong-field tunnel ionization
Bryan, W. A., Frassetto, F., Froud, C. A., Turcu, I. C. E., King, R. B., Calvert, C. R., Nemeth, G. R. A. J., Villoresi, P., Poletto, L., & Springate, E. (2012) · New Journal of Physics · doi:10.1088/1367-2630/14/1/013057 · Cited by 7
Osipov, T., Fang, L., Murphy, B. F., Tarantelli, F., Hosler, E. R., Kukk, E., Bozek, J. D., Bostedt, C., Kanter, E. P., & Berrah, N. (2013) · Journal of Physics B Atomic Molecular and Optical Physics · doi:10.1088/0953-4075/46/16/164032 · Cited by 7
Self-citationKozioł, K., & Rzadkiewicz, J. (2017) · Physical Review A · doi:10.1103/physreva.96.031402 · Cited by 7
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Richard, B., Schäfer, J. M., Jurek, Z., Santra, R., & Inhester, L. (2021) · Journal of Physics B Atomic Molecular and Optical Physics · doi:10.1088/1361-6455/ac2f4f · Cited by 7
Self-citationWhen Diffraction Stops and Destruction Begins
Caleman, C., & Martin, A. V. (2018) · Springer eBooks · doi:10.1007/978-3-030-00551-1_6 · Cited by 7
Interaction of Intense X-Ray Beams with Atoms
Santra, R., & Young, L. (2016) · Springer eBooks · doi:10.1007/978-3-319-14394-1_25 · Cited by 7
Self-citationInvestigation of the Kapitza-Dirac effect in the relativistic regime
Ahrens, S. (2012) · heiDOK (Heidelberg University) · doi:10.11588/heidok.00014049 · Cited by 7
X ‐Ray Emission Spectroscopic Techniques in Bioinorganic Applications
DeBeer, S., & Bergmann, U. (2016) · Wiley eBooks · doi:10.1002/9781119951438.eibc2158 · Cited by 8
Nanometer-Scale Acoustic Wave Packets Generated by Stochastic Core-Level Photoionization Events
Huang, Y., Sun, P., Teitelbaum, S. W., Li, H., Sun, Y., Wang, N., Song, S., Sato, T., Chollet, M., Osaka, T., et al. (2024) · Physical Review X · doi:10.1103/physrevx.14.041010 · Cited by 6
Self-citationObservation of molecular resonant double-core excitation driven by intense X-ray pulses
Pelimanni, E., Fouda, A. E. A., Ho, P. J., Baumann, T., Bokarev, S. I., Fanis, A. D., Dold, S., Grell, G., Ismail, I., Koulentianos, D., et al. (2024) · Communications Physics · doi:10.1038/s42005-024-01804-5 · Cited by 6
Self-citationHarnessing time symmetry to fundamentally alter entanglement in photoionization
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Hard-X-ray Photoelectron Spectroscopy of Atoms and Molecules
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Metadata
- Authors
- Young, L., Kanter, E. P., Krässig, B., Li, Y., March, A. M., Pratt, S. T., Santra, R., Southworth, S. H., Rohringer, N., DiMauro, L. F., Doumy, G., Roedig, C. A., Berrah, N., Fang, L., Hoener, M., Bucksbaum, P. H., Cryan, J. P., Ghimire, S., Glownia, J. M., Reis, D. A., Bozek, J. D., Bostedt, C., & Messerschmidt, M.
- Affiliations
- Argonne National Laboratory (US)
- Lawrence Livermore National Laboratory (US)
- The Ohio State University (US)
- Western Michigan University (US)
- SLAC National Accelerator Laboratory (US)
- Corresponding author
- Young, L.
- ORCID
- Venue
- Nature
- Published
- 2010-07
- Volume
- 466
- Issue
- 7302
- Pages
- 56-61
- ISSN
- 0028-0836 (ISSN-L)
- 1476-4687
- OpenAlex
- W2047732232
- Cited by
- 792
- References
- 54
- Citations by year
- 2026: 14 · 2025: 28 · 2024: 28 · 2023: 29 · 2022: 32 · 2021: 38 · 2020: 55 · 2019: 37 · 2018: 46 · 2017: 39 · 2016: 62 · 2015: 70 · 2014: 67 · 2013: 84 · 2012: 79
- FWCI
- 42.18
- Type
- journal article
- Language
- en
- Open access
- closed
- Licence
- www.springer.com/tdm (tdm)
- Locations
- Nature (publishedVersion)
- PubMed (publishedVersion)
- RePEc: Research Papers in Economics (submittedVersion)
- Desy Publications Database (Deutsches Elektronen-Synchrotron DESY) (submittedVersion)
- European XFEL (submittedVersion)
- Funders
- SLAC National Accelerator Laboratory
- Topics
- Physical Sciences › Physics and Astronomy › Atomic and Molecular Physics, and Optics › Laser-Matter Interactions and Applications
- Physical Sciences › Physics and Astronomy › Atomic and Molecular Physics, and Optics › Atomic and Molecular Physics
- Physical Sciences › Physics and Astronomy › Nuclear and High Energy Physics › Laser-Plasma Interactions and Diagnostics
- Keywords
- X-ray free-electron laser, Linac Coherent Light Source, neon atom, electron stripping, hollow atoms, X-ray transparency, inner-shell vacancies, photoionization, rate equation model, X-ray absorption spectroscopy, X-ray photoelectron spectroscopy, X-ray diffraction
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