The DOI matches its Crossref record; 2 of the 2 references it cites were found in a registry or an index.
Synthesis of ‘unfeasible’ zeolites
Open accessAbstract
Zeolites are porous aluminosilicate materials that have found applications in many different technologies. However, although simulations suggest that there are millions of possible zeolite topologies, only a little over 200 zeolite frameworks of all compositions are currently known, of which about 50 are pure silica materials. This is known as the zeolite conundrum--why have so few of all the possible structures been made? Several criteria have been formulated to explain why most zeolites are unfeasible synthesis targets. Here we demonstrate the synthesis of two such 'unfeasible' zeolites, IPC-9 and IPC-10, through the assembly-disassembly-organization-reassembly mechanism. These new high-silica zeolites have rare characteristics, such as windows that comprise odd-membered rings. Their synthesis opens up the possibility of preparing other zeolites that have not been accessible by traditional solvothermal synthetic methods. We envisage that these findings may lead to a step change in the number and types of zeolites available for future applications.
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Cites
The hydrothermal synthesis of zeolites: Precursors, intermediates and reaction mechanism
Cundy, C. S., & Cox, P. A. (2005) · Microporous and Mesoporous Materials · doi:10.1016/j.micromeso.2005.02.016 · Cited by 1,590
Extra-Large-Pore Zeolites with Two-Dimensional Channels Formed by 14 and 12 Rings
Paillaud, J.-L., Harbuzaru, B., Patarin, J., & Bats, N. (2004) · Science · doi:10.1126/science.1098242 · Cited by 355
Cited by
Post-synthetic modification of covalent organic frameworks
Segura, J. L., Royuela, S., & Mar Ramos, M. (2019) · Chemical Society Reviews · doi:10.1039/c8cs00978c · Cited by 832
Zeolite (In)Stability under Aqueous or Steaming Conditions
Heard, C. J., Grajciar, L., Uhlík, F., Shamzhy, M., Opanasenko, M., Čejka, J., & Nachtigall, P. (2020) · Advanced Materials · doi:10.1002/adma.202003264 · Cited by 157
Self-citationFast room temperature lability of aluminosilicate zeolites
Heard, C. J., Grajciar, L., Rice, C. M., Pugh, S. M., Nachtigall, P., Ashbrook, S. E., & Morris, R. E. (2019) · Nature Communications · doi:10.1038/s41467-019-12752-y · Cited by 121
Self-citationZeolite Synthesis under Nonconventional Conditions: Reagents, Reactors, and Modi Operandi
Deneyer, A., Ke, Q., Devos, J., & Dusselier, M. (2020) · Chemistry of Materials · doi:10.1021/acs.chemmater.9b04741 · Cited by 82
Synthesis and Post‐Synthesis Transformation of Germanosilicate Zeolites
Opanasenko, M., Shamzhy, M., Wang, Y., Yan, W., Nachtigall, P., & Čejka, J. (2020) · Angewandte Chemie International Edition · doi:10.1002/anie.202005776 · Cited by 81
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Metadata
- Authors
- Mazur, M., Wheatley, P. S., Navarro, M., Roth, W. J., Položij, M., Mayoral, A., Eliášová, P., Nachtigall, P., Čejka, J., & Morris, R. E.
- Venue
- Nature Chemistry
- Published
- 2015-10-26
- Volume
- 8
- Issue
- 1
- Pages
- 58-62
- ISSN
- 1755-4330 (ISSN-L)
- 1755-4349
- OpenAlex
- W2209496658
- Cited by
- 228
- References
- 2
- FWCI
- 10.63
- Type
- journal article
- Language
- en
- Open access
- green
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- Mazur, M., Wheatley, P. S., Navarro, M., Roth, W. J., Položij, M., Mayoral, A., Eliášová, P., Nachtigall, P., Čejka, J., & Morris, R. E. (2016). Synthesis of ‘unfeasible’ zeolites. Nature Chemistry. https://doi.org/10.1038/nchem.2374
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